Two-color laser control of photocurrent and high harmonics in graphene

Fuente: arXiv
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Auteurs principaux: Kanega, Minoru, Sato, Masahiro
Format: Preprint
Publié: 2024
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author Kanega, Minoru
Sato, Masahiro
author_facet Kanega, Minoru
Sato, Masahiro
contents We comprehensively investigate two-color-laser-driven photocurrent and high harmonic generation (HHG) in graphene models. By numerically solving the quantum master equation, we uniformly explore a broad parameter regime including both the weak (perturbative) and intense-laser (nonperturbative) cases while considering the dissipation effects. We demonstrate that the HHG spectra can be drastically altered by tuning the real-space path traced by the laser electric field. This controllability is explained by the dynamical symmetry argument. We also show that both the magnitude and the direction of photocurrent (zeroth order harmonics) can be controlled by varying the frequency, intensity, ellipticity, and relative phase of the two-color laser. Furthermore, the nature of photocurrent is shown to be classified into shift- or injection-current types, depending on the phase of two-color laser. Our findings indicate that even in centrosymmetric electron systems, photocurrent and HHG can be quantitatively controlled by adjusting various external parameters if we utilize multicolor laser with a lower spatial or temporal symmetry.
format Preprint
id arxiv_https___arxiv_org_abs_2410_07767
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Two-color laser control of photocurrent and high harmonics in graphene
Kanega, Minoru
Sato, Masahiro
Mesoscale and Nanoscale Physics
Materials Science
Statistical Mechanics
Optics
Quantum Physics
We comprehensively investigate two-color-laser-driven photocurrent and high harmonic generation (HHG) in graphene models. By numerically solving the quantum master equation, we uniformly explore a broad parameter regime including both the weak (perturbative) and intense-laser (nonperturbative) cases while considering the dissipation effects. We demonstrate that the HHG spectra can be drastically altered by tuning the real-space path traced by the laser electric field. This controllability is explained by the dynamical symmetry argument. We also show that both the magnitude and the direction of photocurrent (zeroth order harmonics) can be controlled by varying the frequency, intensity, ellipticity, and relative phase of the two-color laser. Furthermore, the nature of photocurrent is shown to be classified into shift- or injection-current types, depending on the phase of two-color laser. Our findings indicate that even in centrosymmetric electron systems, photocurrent and HHG can be quantitatively controlled by adjusting various external parameters if we utilize multicolor laser with a lower spatial or temporal symmetry.
title Two-color laser control of photocurrent and high harmonics in graphene
topic Mesoscale and Nanoscale Physics
Materials Science
Statistical Mechanics
Optics
Quantum Physics
url https://arxiv.org/abs/2410.07767