Non-bulk Superconductivity in Pr$_4$Ni$_3$O$_{10}$ Single Crystals Under Pressure
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| Main Authors: | , , , , , , , , , , |
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| Format: | Preprint |
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2024
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| _version_ | 1866909348002791424 |
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| author | Chen, Xinglong Poldi, E. H. T. Huyan, Shuyuan Chapai, R. Zheng, H. Budko, S. L. Welp, U. Canfield, P. C. Hemley, Russell J. Mitchell, J. F. Phelan, D. |
| author_facet | Chen, Xinglong Poldi, E. H. T. Huyan, Shuyuan Chapai, R. Zheng, H. Budko, S. L. Welp, U. Canfield, P. C. Hemley, Russell J. Mitchell, J. F. Phelan, D. |
| contents | Magneto-transport measurements of Pr$_4$Ni$_3$O$_{10}$ single crystals performed under externally applied pressures up to 73 GPa in diamond anvil cells with either KBr or Nujol oil as pressure media yield signatures of superconductivity with a maximum onset temperature of approximately 31 K. True zero resistance was not observed, consistent with a non-percolating superconducting volume fraction. Magnetization measurements provided corroborating evidence of superconductivity, with a pressure-dependent diamagnetic signal occurring below the onset temperature, and an estimate from the absolute value of the susceptibility suggests a superconducting volume fraction on the order of 10%. We observe sample-to-sample variations in the magnitude and pressure dependence of Tc as well as a dependence on the configuration of electrical contacts on a given sample. Possible causes of this behavior may be significant inhomogeneities in the pressure and/or damage to the samples induced by the pressure media as well as inhomogeneities in the crystals themselves. The results imply that our as-grown Pr$_4$Ni$_3$O$_{10}$ single crystals are not bulk superconductors but that there is a minority structure present within the crystals that is indeed superconducting. |
| format | Preprint |
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arxiv_https___arxiv_org_abs_2410_10666 |
| institution | arXiv |
| publishDate | 2024 |
| record_format | arxiv |
| spellingShingle | Non-bulk Superconductivity in Pr$_4$Ni$_3$O$_{10}$ Single Crystals Under Pressure Chen, Xinglong Poldi, E. H. T. Huyan, Shuyuan Chapai, R. Zheng, H. Budko, S. L. Welp, U. Canfield, P. C. Hemley, Russell J. Mitchell, J. F. Phelan, D. Superconductivity Materials Science Magneto-transport measurements of Pr$_4$Ni$_3$O$_{10}$ single crystals performed under externally applied pressures up to 73 GPa in diamond anvil cells with either KBr or Nujol oil as pressure media yield signatures of superconductivity with a maximum onset temperature of approximately 31 K. True zero resistance was not observed, consistent with a non-percolating superconducting volume fraction. Magnetization measurements provided corroborating evidence of superconductivity, with a pressure-dependent diamagnetic signal occurring below the onset temperature, and an estimate from the absolute value of the susceptibility suggests a superconducting volume fraction on the order of 10%. We observe sample-to-sample variations in the magnitude and pressure dependence of Tc as well as a dependence on the configuration of electrical contacts on a given sample. Possible causes of this behavior may be significant inhomogeneities in the pressure and/or damage to the samples induced by the pressure media as well as inhomogeneities in the crystals themselves. The results imply that our as-grown Pr$_4$Ni$_3$O$_{10}$ single crystals are not bulk superconductors but that there is a minority structure present within the crystals that is indeed superconducting. |
| title | Non-bulk Superconductivity in Pr$_4$Ni$_3$O$_{10}$ Single Crystals Under Pressure |
| topic | Superconductivity Materials Science |
| url | https://arxiv.org/abs/2410.10666 |