Electronic Raman scattering of antiferromagnetic excitonic insulators

Fuente: arXiv
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Auteurs principaux: Suwa, Hidemaro, Zhang, Shang-Shun, Batista, Cristian D.
Format: Preprint
Publié: 2024
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author Suwa, Hidemaro
Zhang, Shang-Shun
Batista, Cristian D.
author_facet Suwa, Hidemaro
Zhang, Shang-Shun
Batista, Cristian D.
contents The excitonic insulator, a quantum mechanical state arising from exciton condensation, was proposed theoretically many years ago but has yet to be experimentally confirmed. The discovery of correlated transition metal oxides based on $4d$ and $5d$ elements, where the on-site Coulomb repulsion is comparable to the dominant hopping amplitude, presents a unique opportunity to study exciton condensation. By constructing an effective mean field Raman operator for the Hubbard model, we derive the low-energy electronic Raman scattering cross section, demonstrating Raman spectroscopy as a powerful tool for detecting exciton condensation. Here, we demonstrate that Raman scattering directly reveals exciton condensation in the bilayer iridate Sr$_3$Ir$_2$O$_7$ under pressure.
format Preprint
id arxiv_https___arxiv_org_abs_2410_13715
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Electronic Raman scattering of antiferromagnetic excitonic insulators
Suwa, Hidemaro
Zhang, Shang-Shun
Batista, Cristian D.
Strongly Correlated Electrons
The excitonic insulator, a quantum mechanical state arising from exciton condensation, was proposed theoretically many years ago but has yet to be experimentally confirmed. The discovery of correlated transition metal oxides based on $4d$ and $5d$ elements, where the on-site Coulomb repulsion is comparable to the dominant hopping amplitude, presents a unique opportunity to study exciton condensation. By constructing an effective mean field Raman operator for the Hubbard model, we derive the low-energy electronic Raman scattering cross section, demonstrating Raman spectroscopy as a powerful tool for detecting exciton condensation. Here, we demonstrate that Raman scattering directly reveals exciton condensation in the bilayer iridate Sr$_3$Ir$_2$O$_7$ under pressure.
title Electronic Raman scattering of antiferromagnetic excitonic insulators
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2410.13715