Interplay of electron-phonon coupling, pseudogap, and superconductivity in CsCa$_2$Fe$_4$As$_4$F$_2$ studied using ultrafast optical spectroscopy

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Hauptverfasser: Wu, Qi-Yi, Zhang, Chen, Li, Bai-Zhuo, Liu, Hao, Song, Jiao-Jiao, Chen, Bo, Liu, Hai-Yun, Duan, Yu-Xia, He, Jun, Liu, Jun, Cao, Guang-Han, Meng, Jian-Qiao
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Veröffentlicht: 2024
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author Wu, Qi-Yi
Zhang, Chen
Li, Bai-Zhuo
Liu, Hao
Song, Jiao-Jiao
Chen, Bo
Liu, Hai-Yun
Duan, Yu-Xia
He, Jun
Liu, Jun
Cao, Guang-Han
Meng, Jian-Qiao
author_facet Wu, Qi-Yi
Zhang, Chen
Li, Bai-Zhuo
Liu, Hao
Song, Jiao-Jiao
Chen, Bo
Liu, Hai-Yun
Duan, Yu-Xia
He, Jun
Liu, Jun
Cao, Guang-Han
Meng, Jian-Qiao
contents The quasiparticle relaxation dynamics of the iron-based superconductor CsCa$_2$Fe$_4$As$_4$F$_2$ ($T_c$ $\sim$ 29 K) were investigated using ultrafast optical spectroscopy. A pseudogap ($Δ_{PG}$ $\approx$ 3.3 meV) was observed to open below $T^{\ast}$ $\approx$ 60 K, prior to the emergence of a superconducting gap ($Δ$ $\approx$ 6.6 $\pm$ 0.4 meV). At high excitation fluence, a coherent A1g phonon mode at 5.49 THz was identified, exhibiting deviations from anharmonic behavior below $T_c$. The electron-phonon coupling constant for this mode was estimated to be $λ_{A_{1g}}$ $\approx$ 0.23. These results provide insights into the interplay between the electron-phonon interactions, pseudogap, and the superconducting pairing mechanism in CsCa$_2$Fe$_4$As$_4$F$_2$.
format Preprint
id arxiv_https___arxiv_org_abs_2410_16610
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Interplay of electron-phonon coupling, pseudogap, and superconductivity in CsCa$_2$Fe$_4$As$_4$F$_2$ studied using ultrafast optical spectroscopy
Wu, Qi-Yi
Zhang, Chen
Li, Bai-Zhuo
Liu, Hao
Song, Jiao-Jiao
Chen, Bo
Liu, Hai-Yun
Duan, Yu-Xia
He, Jun
Liu, Jun
Cao, Guang-Han
Meng, Jian-Qiao
Superconductivity
The quasiparticle relaxation dynamics of the iron-based superconductor CsCa$_2$Fe$_4$As$_4$F$_2$ ($T_c$ $\sim$ 29 K) were investigated using ultrafast optical spectroscopy. A pseudogap ($Δ_{PG}$ $\approx$ 3.3 meV) was observed to open below $T^{\ast}$ $\approx$ 60 K, prior to the emergence of a superconducting gap ($Δ$ $\approx$ 6.6 $\pm$ 0.4 meV). At high excitation fluence, a coherent A1g phonon mode at 5.49 THz was identified, exhibiting deviations from anharmonic behavior below $T_c$. The electron-phonon coupling constant for this mode was estimated to be $λ_{A_{1g}}$ $\approx$ 0.23. These results provide insights into the interplay between the electron-phonon interactions, pseudogap, and the superconducting pairing mechanism in CsCa$_2$Fe$_4$As$_4$F$_2$.
title Interplay of electron-phonon coupling, pseudogap, and superconductivity in CsCa$_2$Fe$_4$As$_4$F$_2$ studied using ultrafast optical spectroscopy
topic Superconductivity
url https://arxiv.org/abs/2410.16610