Quantum versus semi-classical signatures of correlated triple ionization in Dalitz plots

Fuente: arXiv
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Main Authors: Efimov, Dmitry K., Katsoulis, Georgios P., Rozpętkowski, Tymoteusz, Chwałowski, Sergiusz, Emmanouilidou, Agapi, Prauzner-Bechcicki, Jakub S.
Format: Preprint
Published: 2024
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author Efimov, Dmitry K.
Katsoulis, Georgios P.
Rozpętkowski, Tymoteusz
Chwałowski, Sergiusz
Emmanouilidou, Agapi
Prauzner-Bechcicki, Jakub S.
author_facet Efimov, Dmitry K.
Katsoulis, Georgios P.
Rozpętkowski, Tymoteusz
Chwałowski, Sergiusz
Emmanouilidou, Agapi
Prauzner-Bechcicki, Jakub S.
contents We investigate correlated three-electron escape in Ne when driven by an intense, infrared laser field. We do so by employing a reduced-dimensionality quantum-mechanical model and two three-dimensional semi-classical models. One semi-classical model is a recently developed one that accounts with effective coulomb potentials for the interaction between two bound electrons (ECBB) while it fully accounts for all other interactions. The other semi-classical model is the Heisenberg one, which effectively accounts for the interaction of each electron with the core via a soft-core potential. We identify and compare the signatures of correlated three-electron escape for both quantum and semi-classical models on Dalitz plots and find a better agreement between the quantum and the ECBB model. We also show that a central ``spot'' on the Dalitz plots is reproduced by all models. Using the ECBB model we associate this ``spot'' with the direct triple ionization pathway and argue this to be the case also for the quantum model. Devising a simple classical model that accounts for the direct pathway of triple ionization, we show that the width of this spot in the Dalitz plots solely depends on the time of tunnel-ionization.
format Preprint
id arxiv_https___arxiv_org_abs_2410_16797
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Quantum versus semi-classical signatures of correlated triple ionization in Dalitz plots
Efimov, Dmitry K.
Katsoulis, Georgios P.
Rozpętkowski, Tymoteusz
Chwałowski, Sergiusz
Emmanouilidou, Agapi
Prauzner-Bechcicki, Jakub S.
Atomic Physics
We investigate correlated three-electron escape in Ne when driven by an intense, infrared laser field. We do so by employing a reduced-dimensionality quantum-mechanical model and two three-dimensional semi-classical models. One semi-classical model is a recently developed one that accounts with effective coulomb potentials for the interaction between two bound electrons (ECBB) while it fully accounts for all other interactions. The other semi-classical model is the Heisenberg one, which effectively accounts for the interaction of each electron with the core via a soft-core potential. We identify and compare the signatures of correlated three-electron escape for both quantum and semi-classical models on Dalitz plots and find a better agreement between the quantum and the ECBB model. We also show that a central ``spot'' on the Dalitz plots is reproduced by all models. Using the ECBB model we associate this ``spot'' with the direct triple ionization pathway and argue this to be the case also for the quantum model. Devising a simple classical model that accounts for the direct pathway of triple ionization, we show that the width of this spot in the Dalitz plots solely depends on the time of tunnel-ionization.
title Quantum versus semi-classical signatures of correlated triple ionization in Dalitz plots
topic Atomic Physics
url https://arxiv.org/abs/2410.16797