Positive oscillating magnetoresistance in a van der Waals antiferromagnetic semiconductor

Fuente: arXiv
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Main Authors: Lin, Xiaohanwen, WU, Fan, Ubrig, Nicolas, Liao, Menghan, Yao, Fengrui, Gutiérrez-Lezama, Ignacio, Morpurgo, Alberto F.
Format: Preprint
Published: 2024
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author Lin, Xiaohanwen
WU, Fan
Ubrig, Nicolas
Liao, Menghan
Yao, Fengrui
Gutiérrez-Lezama, Ignacio
Morpurgo, Alberto F.
author_facet Lin, Xiaohanwen
WU, Fan
Ubrig, Nicolas
Liao, Menghan
Yao, Fengrui
Gutiérrez-Lezama, Ignacio
Morpurgo, Alberto F.
contents In all van der Waals layered antiferromagnetic semiconductors investigated so far a negative magnetoresistance has been observed in vertical transport measurements, with characteristic trends that do not depend on applied bias. Here we report vertical transport measurements on layered antiferromagnetic semiconductor CrPS$_4$ that exhibit a drastically different behavior, namely a strongly bias dependent, positive magnetoresistance that is accompanied by pronounced oscillations for devices whose thickness is smaller than 10 nm. We establish that this unexpected behavior originates from transport being space-charge limited, and not injection limited as for layered antiferromagetic semiconductors studid earlier. Our analysis indicates that the positive magnetoresistance and the oscillations only occur when electrons are injected into in-gap defect states, whereas when electrons are injected into the conduction band the magnetoresistance vanishes. We propose a microscopic explanation for the observed phenomena that combines concepts typical of transport through disordered semiconductors with known properties of the CrPS$_4$ magnetic state, which captures all basic experimental observations. Our results illustrate the need to understand in detail the nature of transport through vdW magnets, to extract information about the nature of the order magnetic states and its microscopic properties.
format Preprint
id arxiv_https___arxiv_org_abs_2410_17930
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Positive oscillating magnetoresistance in a van der Waals antiferromagnetic semiconductor
Lin, Xiaohanwen
WU, Fan
Ubrig, Nicolas
Liao, Menghan
Yao, Fengrui
Gutiérrez-Lezama, Ignacio
Morpurgo, Alberto F.
Mesoscale and Nanoscale Physics
Disordered Systems and Neural Networks
Materials Science
In all van der Waals layered antiferromagnetic semiconductors investigated so far a negative magnetoresistance has been observed in vertical transport measurements, with characteristic trends that do not depend on applied bias. Here we report vertical transport measurements on layered antiferromagnetic semiconductor CrPS$_4$ that exhibit a drastically different behavior, namely a strongly bias dependent, positive magnetoresistance that is accompanied by pronounced oscillations for devices whose thickness is smaller than 10 nm. We establish that this unexpected behavior originates from transport being space-charge limited, and not injection limited as for layered antiferromagetic semiconductors studid earlier. Our analysis indicates that the positive magnetoresistance and the oscillations only occur when electrons are injected into in-gap defect states, whereas when electrons are injected into the conduction band the magnetoresistance vanishes. We propose a microscopic explanation for the observed phenomena that combines concepts typical of transport through disordered semiconductors with known properties of the CrPS$_4$ magnetic state, which captures all basic experimental observations. Our results illustrate the need to understand in detail the nature of transport through vdW magnets, to extract information about the nature of the order magnetic states and its microscopic properties.
title Positive oscillating magnetoresistance in a van der Waals antiferromagnetic semiconductor
topic Mesoscale and Nanoscale Physics
Disordered Systems and Neural Networks
Materials Science
url https://arxiv.org/abs/2410.17930