Enhanced laser-induced single-cycle terahertz generation in a spintronic emitter with a gradient interface

Fuente: arXiv
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Autori principali: Shelukhin, L. A., Kuzikova, A. V., Telegin, A. V., Bessonov, V. D., Ognev, A. V., Samardak, A. S., Park, Junho, Kim, Young Keun, Kalashnikova, A. M.
Natura: Preprint
Pubblicazione: 2024
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author Shelukhin, L. A.
Kuzikova, A. V.
Telegin, A. V.
Bessonov, V. D.
Ognev, A. V.
Samardak, A. S.
Park, Junho
Kim, Young Keun
Kalashnikova, A. M.
author_facet Shelukhin, L. A.
Kuzikova, A. V.
Telegin, A. V.
Bessonov, V. D.
Ognev, A. V.
Samardak, A. S.
Park, Junho
Kim, Young Keun
Kalashnikova, A. M.
contents The development of spintronic emitters of broadband THz pulses relies on designing heterostructures where processes of laser-driven spin current generation and subsequent spin-to-charge current conversion are the most efficient. An interface between ferromagnetic and nonmagnetic layers in the emitter is one of the critical elements. Here, we study experimentally single-cycle THz pulse generation from a laser-pulse excited Pt/Co emitter with a composition gradient interface between Pt and Co and compare it with the emission from a conventional Pt/Co structure with an abrupt interface. We find that the gradient interface enhances the efficiency of optics-to-THz conversion by a factor of two in a wide range of optical fluences up to 3 mJ cm$^{-2}$. We reveal that this enhancement is caused by a pronounced increase in transmittance of the laser-driven spin-polarized current through the gradient interface compared to the abrupt one. Furthermore, we find that such a transmission deteriorates with laser fluence due to the spin accumulation effect.
format Preprint
id arxiv_https___arxiv_org_abs_2410_18591
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Enhanced laser-induced single-cycle terahertz generation in a spintronic emitter with a gradient interface
Shelukhin, L. A.
Kuzikova, A. V.
Telegin, A. V.
Bessonov, V. D.
Ognev, A. V.
Samardak, A. S.
Park, Junho
Kim, Young Keun
Kalashnikova, A. M.
Applied Physics
Mesoscale and Nanoscale Physics
Materials Science
The development of spintronic emitters of broadband THz pulses relies on designing heterostructures where processes of laser-driven spin current generation and subsequent spin-to-charge current conversion are the most efficient. An interface between ferromagnetic and nonmagnetic layers in the emitter is one of the critical elements. Here, we study experimentally single-cycle THz pulse generation from a laser-pulse excited Pt/Co emitter with a composition gradient interface between Pt and Co and compare it with the emission from a conventional Pt/Co structure with an abrupt interface. We find that the gradient interface enhances the efficiency of optics-to-THz conversion by a factor of two in a wide range of optical fluences up to 3 mJ cm$^{-2}$. We reveal that this enhancement is caused by a pronounced increase in transmittance of the laser-driven spin-polarized current through the gradient interface compared to the abrupt one. Furthermore, we find that such a transmission deteriorates with laser fluence due to the spin accumulation effect.
title Enhanced laser-induced single-cycle terahertz generation in a spintronic emitter with a gradient interface
topic Applied Physics
Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2410.18591