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Main Authors: Ozawa, Keisuke, Sugimoto, Hiroshi, Shima, Daisuke, Hinamoto, Tatsuki, Habil, Mojtaba Karimi, Lee, Yan Joe, Raza, Søren, Imaeda, Keisuke, Ueno, Kosei, Brongersma, Mark L., Fujii, Minoru
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2410.20743
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author Ozawa, Keisuke
Sugimoto, Hiroshi
Shima, Daisuke
Hinamoto, Tatsuki
Habil, Mojtaba Karimi
Lee, Yan Joe
Raza, Søren
Imaeda, Keisuke
Ueno, Kosei
Brongersma, Mark L.
Fujii, Minoru
author_facet Ozawa, Keisuke
Sugimoto, Hiroshi
Shima, Daisuke
Hinamoto, Tatsuki
Habil, Mojtaba Karimi
Lee, Yan Joe
Raza, Søren
Imaeda, Keisuke
Ueno, Kosei
Brongersma, Mark L.
Fujii, Minoru
contents A dielectric Mie-resonant nanoantenna is capable of controlling the directionality of the emission from nearby quantum emitters through the excitation of multiple degenerate Mie resonances. A crystalline silicon nanosphere (Si NS) is a promising candidate for a dielectric nanoantenna because crystalline Si has a large refractive index (3.8 at 650 nm) and the small imaginary part of a complex refractive index (0.015 at 650 nm) as an optical material. In this work, we control the emission directionality of excitons supported by monolayer transition metal dichalcogenides (1L-TMDCs) using a Si NS. We first discuss the condition to extract the emission preferentially towards the Si NS side from the analytical calculations. We then study the photoluminescence (PL) of 1L-TMDCs on which differently sized single Si NSs are placed. We show that the PL spectral shape strongly depends on the emission direction, and that the emission toward the Si NS side (top) with respect to the opposite side (bottom) is the largest at wavelengths between the magnetic dipole and electric dipole Mie resonances of a Si NS. Finally, we quantitatively discuss the spectral shape of the top-to-bottom ratio from numerical simulations.
format Preprint
id arxiv_https___arxiv_org_abs_2410_20743
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Routing Light Emission from Monolayer MoS$_2$ by Mie Resonances of Crystalline Silicon Nanospheres
Ozawa, Keisuke
Sugimoto, Hiroshi
Shima, Daisuke
Hinamoto, Tatsuki
Habil, Mojtaba Karimi
Lee, Yan Joe
Raza, Søren
Imaeda, Keisuke
Ueno, Kosei
Brongersma, Mark L.
Fujii, Minoru
Optics
Mesoscale and Nanoscale Physics
A dielectric Mie-resonant nanoantenna is capable of controlling the directionality of the emission from nearby quantum emitters through the excitation of multiple degenerate Mie resonances. A crystalline silicon nanosphere (Si NS) is a promising candidate for a dielectric nanoantenna because crystalline Si has a large refractive index (3.8 at 650 nm) and the small imaginary part of a complex refractive index (0.015 at 650 nm) as an optical material. In this work, we control the emission directionality of excitons supported by monolayer transition metal dichalcogenides (1L-TMDCs) using a Si NS. We first discuss the condition to extract the emission preferentially towards the Si NS side from the analytical calculations. We then study the photoluminescence (PL) of 1L-TMDCs on which differently sized single Si NSs are placed. We show that the PL spectral shape strongly depends on the emission direction, and that the emission toward the Si NS side (top) with respect to the opposite side (bottom) is the largest at wavelengths between the magnetic dipole and electric dipole Mie resonances of a Si NS. Finally, we quantitatively discuss the spectral shape of the top-to-bottom ratio from numerical simulations.
title Routing Light Emission from Monolayer MoS$_2$ by Mie Resonances of Crystalline Silicon Nanospheres
topic Optics
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2410.20743