Observation of chiral domain walls in an octupole-ordered antiferromagnet

Fuente: arXiv
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Main Authors: Tsukamoto, Moeta, Xu, Zhewen, Higo, Tomoya, Kondou, Kouta, Sasaki, Kento, Asakura, Mihiro, Sakamoto, Shoya, Gambardella, Pietro, Miwa, Shinji, Otani, YoshiChika, Nakatsuji, Satoru, Degen, Christian L., Kobayashi, Kensuke
Format: Preprint
Published: 2024
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author Tsukamoto, Moeta
Xu, Zhewen
Higo, Tomoya
Kondou, Kouta
Sasaki, Kento
Asakura, Mihiro
Sakamoto, Shoya
Gambardella, Pietro
Miwa, Shinji
Otani, YoshiChika
Nakatsuji, Satoru
Degen, Christian L.
Kobayashi, Kensuke
author_facet Tsukamoto, Moeta
Xu, Zhewen
Higo, Tomoya
Kondou, Kouta
Sasaki, Kento
Asakura, Mihiro
Sakamoto, Shoya
Gambardella, Pietro
Miwa, Shinji
Otani, YoshiChika
Nakatsuji, Satoru
Degen, Christian L.
Kobayashi, Kensuke
contents Spin chirality in antiferromagnets offers new opportunities for spintronics. The kagome antiferromagnet Mn3Sn is a paradigmatic material in which the antiferromagnetic order parameter can be detected and controlled by electrical means. However, direct investigation of the magnetic texture of Mn3Sn has been challenging because of the tiny moment hosted in its magnetic octupole, hindering further clarification of this unique material. Here, we address this issue by observing the stray magnetic field from Mn3Sn using a diamond quantum scanning magnetometer. The spatially-resolved intrinsic domains and domain walls in a high-quality single-crystalline Mn3Sn film quantitatively reveal the polarization angle of the magnetic octupole in the kagome plane, the domain's local magnetization, the domain wall's width and chirality, and the octupole order in domain walls. Our nanoscale investigation of Mn3Sn, a powerful complement to macroscopic measurements, paves the road for developing chiral antiferromagnetism and its potential for spintronic applications.
format Preprint
id arxiv_https___arxiv_org_abs_2410_23607
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Observation of chiral domain walls in an octupole-ordered antiferromagnet
Tsukamoto, Moeta
Xu, Zhewen
Higo, Tomoya
Kondou, Kouta
Sasaki, Kento
Asakura, Mihiro
Sakamoto, Shoya
Gambardella, Pietro
Miwa, Shinji
Otani, YoshiChika
Nakatsuji, Satoru
Degen, Christian L.
Kobayashi, Kensuke
Materials Science
Mesoscale and Nanoscale Physics
Spin chirality in antiferromagnets offers new opportunities for spintronics. The kagome antiferromagnet Mn3Sn is a paradigmatic material in which the antiferromagnetic order parameter can be detected and controlled by electrical means. However, direct investigation of the magnetic texture of Mn3Sn has been challenging because of the tiny moment hosted in its magnetic octupole, hindering further clarification of this unique material. Here, we address this issue by observing the stray magnetic field from Mn3Sn using a diamond quantum scanning magnetometer. The spatially-resolved intrinsic domains and domain walls in a high-quality single-crystalline Mn3Sn film quantitatively reveal the polarization angle of the magnetic octupole in the kagome plane, the domain's local magnetization, the domain wall's width and chirality, and the octupole order in domain walls. Our nanoscale investigation of Mn3Sn, a powerful complement to macroscopic measurements, paves the road for developing chiral antiferromagnetism and its potential for spintronic applications.
title Observation of chiral domain walls in an octupole-ordered antiferromagnet
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2410.23607