Laser-driven cold-field emission source for ultrafast transmission electron microscopy

Fuente: arXiv
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Auteurs principaux: Schröder, Alexander, Wendeln, Andreas, Weber, Jonathan T., Mukai, Masaki, Kohno, Yuji, Schäfer, Sascha
Format: Preprint
Publié: 2024
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author Schröder, Alexander
Wendeln, Andreas
Weber, Jonathan T.
Mukai, Masaki
Kohno, Yuji
Schäfer, Sascha
author_facet Schröder, Alexander
Wendeln, Andreas
Weber, Jonathan T.
Mukai, Masaki
Kohno, Yuji
Schäfer, Sascha
contents Ultrafast transmission electron microscopy (UTEM) has emerged as a versatile technique for the time-resolved imaging of nanoscale dynamics on timescales down to few-hundred attoseconds but the temporal and spatial resolutions are still limited by the coherence properties of pulsed electron sources. Here, we report the development of a novel laser-driven linear cold-field electron emitter integrated in a state-of-the-art UTEM system. Illuminating the sharp tungsten emitter tip with a UV light pulse generates ultrashort femtosecond electron pulses of 220 fs pulse duration, with energy widths as low as 360 meV. The photoelectron emitter demonstrates exceptional spatial coherence, achieving focal spot sizes down to 2 $\mathring {\mathrm A}$ and a peak normalized brightness exceeding 6.7 $\times 10^{13}$ A/m$^2$sr. With an order-of-magnitude improvement compared to previously employed laser-driven Schottky field emitters, the present development opens up the field of ultrafast atomic-scale electron probing.
format Preprint
id arxiv_https___arxiv_org_abs_2410_23961
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Laser-driven cold-field emission source for ultrafast transmission electron microscopy
Schröder, Alexander
Wendeln, Andreas
Weber, Jonathan T.
Mukai, Masaki
Kohno, Yuji
Schäfer, Sascha
Instrumentation and Detectors
Mesoscale and Nanoscale Physics
Ultrafast transmission electron microscopy (UTEM) has emerged as a versatile technique for the time-resolved imaging of nanoscale dynamics on timescales down to few-hundred attoseconds but the temporal and spatial resolutions are still limited by the coherence properties of pulsed electron sources. Here, we report the development of a novel laser-driven linear cold-field electron emitter integrated in a state-of-the-art UTEM system. Illuminating the sharp tungsten emitter tip with a UV light pulse generates ultrashort femtosecond electron pulses of 220 fs pulse duration, with energy widths as low as 360 meV. The photoelectron emitter demonstrates exceptional spatial coherence, achieving focal spot sizes down to 2 $\mathring {\mathrm A}$ and a peak normalized brightness exceeding 6.7 $\times 10^{13}$ A/m$^2$sr. With an order-of-magnitude improvement compared to previously employed laser-driven Schottky field emitters, the present development opens up the field of ultrafast atomic-scale electron probing.
title Laser-driven cold-field emission source for ultrafast transmission electron microscopy
topic Instrumentation and Detectors
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2410.23961