In-situ Self-optimization of Quantum Dot Emission for Lasers by Machine-Learning Assisted Epitaxy

Fuente: arXiv
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Main Authors: Shen, Chao, Zhan, Wenkang, Pan, Shujie, Hao, Hongyue, Zhuo, Ning, Xin, Kaiyao, Cong, Hui, Xu, Chi, Xu, Bo, Ng, Tien Khee, Chen, Siming, Xue, Chunlai, Liu, Fengqi, Wang, Zhanguo, Zhao, Chao
Format: Preprint
Published: 2024
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author Shen, Chao
Zhan, Wenkang
Pan, Shujie
Hao, Hongyue
Zhuo, Ning
Xin, Kaiyao
Cong, Hui
Xu, Chi
Xu, Bo
Ng, Tien Khee
Chen, Siming
Xue, Chunlai
Liu, Fengqi
Wang, Zhanguo
Zhao, Chao
author_facet Shen, Chao
Zhan, Wenkang
Pan, Shujie
Hao, Hongyue
Zhuo, Ning
Xin, Kaiyao
Cong, Hui
Xu, Chi
Xu, Bo
Ng, Tien Khee
Chen, Siming
Xue, Chunlai
Liu, Fengqi
Wang, Zhanguo
Zhao, Chao
contents Traditional methods for optimizing light source emissions rely on a time-consuming trial-and-error approach. While in-situ optimization of light source gain media emission during growth is ideal, it has yet to be realized. In this work, we integrate in-situ reflection high-energy electron diffraction (RHEED) with machine learning (ML) to correlate the surface reconstruction with the photoluminescence (PL) of InAs/GaAs quantum dots (QDs), which serve as the active region of lasers. A lightweight ResNet-GLAM model is employed for the real-time processing of RHEED data as input, enabling effective identification of optical performance. This approach guides the dynamic optimization of growth parameters, allowing real-time feedback control to adjust the QDs emission for lasers. We successfully optimized InAs QDs on GaAs substrates, with a 3.2-fold increase in PL intensity and a reduction in full width at half maximum (FWHM) from 36.69 meV to 28.17 meV under initially suboptimal growth conditions. Our automated, in-situ self-optimized lasers with 5-layer InAs QDs achieved electrically pumped continuous-wave operation at 1240 nm with a low threshold current of 150 A/cm2 at room temperature, an excellent performance comparable to samples grown through traditional manual multi-parameter optimization methods. These results mark a significant step toward intelligent, low-cost, and reproductive light emitters production.
format Preprint
id arxiv_https___arxiv_org_abs_2411_00332
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle In-situ Self-optimization of Quantum Dot Emission for Lasers by Machine-Learning Assisted Epitaxy
Shen, Chao
Zhan, Wenkang
Pan, Shujie
Hao, Hongyue
Zhuo, Ning
Xin, Kaiyao
Cong, Hui
Xu, Chi
Xu, Bo
Ng, Tien Khee
Chen, Siming
Xue, Chunlai
Liu, Fengqi
Wang, Zhanguo
Zhao, Chao
Mesoscale and Nanoscale Physics
Machine Learning
Traditional methods for optimizing light source emissions rely on a time-consuming trial-and-error approach. While in-situ optimization of light source gain media emission during growth is ideal, it has yet to be realized. In this work, we integrate in-situ reflection high-energy electron diffraction (RHEED) with machine learning (ML) to correlate the surface reconstruction with the photoluminescence (PL) of InAs/GaAs quantum dots (QDs), which serve as the active region of lasers. A lightweight ResNet-GLAM model is employed for the real-time processing of RHEED data as input, enabling effective identification of optical performance. This approach guides the dynamic optimization of growth parameters, allowing real-time feedback control to adjust the QDs emission for lasers. We successfully optimized InAs QDs on GaAs substrates, with a 3.2-fold increase in PL intensity and a reduction in full width at half maximum (FWHM) from 36.69 meV to 28.17 meV under initially suboptimal growth conditions. Our automated, in-situ self-optimized lasers with 5-layer InAs QDs achieved electrically pumped continuous-wave operation at 1240 nm with a low threshold current of 150 A/cm2 at room temperature, an excellent performance comparable to samples grown through traditional manual multi-parameter optimization methods. These results mark a significant step toward intelligent, low-cost, and reproductive light emitters production.
title In-situ Self-optimization of Quantum Dot Emission for Lasers by Machine-Learning Assisted Epitaxy
topic Mesoscale and Nanoscale Physics
Machine Learning
url https://arxiv.org/abs/2411.00332