Exploiting the Variational Quantum Eigensolver for Determining Ground State Energy of Protocatechuic Acid

Fuente: arXiv
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Main Authors: de Jesus, Gleydson Fernandes, Teixeira, Erico Souza, Galvão, Lucas Queiroz, da Silva, Maria Heloísa Fraga, Neto, Mauro Queiroz Nooblath, Fernandez, Bruno Oziel, Cruz, Clebson dos Santos
Format: Preprint
Published: 2024
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author de Jesus, Gleydson Fernandes
Teixeira, Erico Souza
Galvão, Lucas Queiroz
da Silva, Maria Heloísa Fraga
Neto, Mauro Queiroz Nooblath
Fernandez, Bruno Oziel
Cruz, Clebson dos Santos
author_facet de Jesus, Gleydson Fernandes
Teixeira, Erico Souza
Galvão, Lucas Queiroz
da Silva, Maria Heloísa Fraga
Neto, Mauro Queiroz Nooblath
Fernandez, Bruno Oziel
Cruz, Clebson dos Santos
contents The Variational Quantum Eigensolver (VQE) is a promising hybrid algorithm, utilizing both quantum and classical computers to obtain the ground state energy of molecules. In this context, this study applies VQE to investigate the ground state of protocatechuic acid, analyzing its performance with various Ansätze and active spaces. Subsequently, all VQE results were compared to those obtained with the Hartree-Fock (HF) method. The results demonstrate that Ansätze, like unitary coupled-cluster singles and doubles (UCCSD) and variations of Hardware-Efficient, generally achieve accuracy close to that of HF. Furthermore, the increase in active space has led to the models becoming more difficult to converge to values with a greater distance from the correct energy. In summary, the findings of this study reinforce the use of VQE as a powerful tool for analyzing molecular ground state energies. Finally, the results underscore the critical importance of Ansatz selection and active space size in VQE performance, providing valuable insights into its potential and limitations.
format Preprint
id arxiv_https___arxiv_org_abs_2411_00990
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Exploiting the Variational Quantum Eigensolver for Determining Ground State Energy of Protocatechuic Acid
de Jesus, Gleydson Fernandes
Teixeira, Erico Souza
Galvão, Lucas Queiroz
da Silva, Maria Heloísa Fraga
Neto, Mauro Queiroz Nooblath
Fernandez, Bruno Oziel
Cruz, Clebson dos Santos
Chemical Physics
Materials Science
Quantum Physics
The Variational Quantum Eigensolver (VQE) is a promising hybrid algorithm, utilizing both quantum and classical computers to obtain the ground state energy of molecules. In this context, this study applies VQE to investigate the ground state of protocatechuic acid, analyzing its performance with various Ansätze and active spaces. Subsequently, all VQE results were compared to those obtained with the Hartree-Fock (HF) method. The results demonstrate that Ansätze, like unitary coupled-cluster singles and doubles (UCCSD) and variations of Hardware-Efficient, generally achieve accuracy close to that of HF. Furthermore, the increase in active space has led to the models becoming more difficult to converge to values with a greater distance from the correct energy. In summary, the findings of this study reinforce the use of VQE as a powerful tool for analyzing molecular ground state energies. Finally, the results underscore the critical importance of Ansatz selection and active space size in VQE performance, providing valuable insights into its potential and limitations.
title Exploiting the Variational Quantum Eigensolver for Determining Ground State Energy of Protocatechuic Acid
topic Chemical Physics
Materials Science
Quantum Physics
url https://arxiv.org/abs/2411.00990