Trion Engineered Multimodal Transistors in Two dimensional Bilayer Semiconductor Lateral Heterostructures

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Main Authors: Kundu, Baisali, Chakrabarty, Poulomi, Dhara, Avijit, Rosati, Roberto, Samanta, Chandan, Chakraborty, Suman K., Sahoo, Srilagna, Dhara, Sajal, Dash, Saroj P., Malic, Ermin, Lodha, Saurabh, Sahoo, Prasana K.
Format: Preprint
Published: 2024
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author Kundu, Baisali
Chakrabarty, Poulomi
Dhara, Avijit
Rosati, Roberto
Samanta, Chandan
Chakraborty, Suman K.
Sahoo, Srilagna
Dhara, Sajal
Dash, Saroj P.
Malic, Ermin
Lodha, Saurabh
Sahoo, Prasana K.
author_facet Kundu, Baisali
Chakrabarty, Poulomi
Dhara, Avijit
Rosati, Roberto
Samanta, Chandan
Chakraborty, Suman K.
Sahoo, Srilagna
Dhara, Sajal
Dash, Saroj P.
Malic, Ermin
Lodha, Saurabh
Sahoo, Prasana K.
contents Multimodal device operations are essential to advancing the integration of 2D semiconductors in electronics, photonics, information and quantum technology. Precise control over carrier dynamics, particularly exciton generation and transport, is crucial for finetuning the functionality of optoelectronic devices based on 2D semiconductor heterostructure. However, the traditional exciton engineering methods in 2D semiconductors are mainly restricted to the artificially assembled vertical pn heterostructures with electrical or strain induced confinements. In this study, we utilized bilayer 2D lateral npn multijunction heterostructures with intrinsically spatially separated energy landscapes to achieve preferential exciton generation and manipulation without external confinement. In lateral npn FET geometry, we uncover unique and nontrivial properties, including dynamic tuning of channel photoresponsivity from positive to negative. The multimodal operation of these 2D FETs is achieved by carefully adjusting electrical bias and the impinging photon energy, enabling precise control over the trions generation and transport. Cryogenic photoluminescence measurement revealed the presence of trions in bilayer MoSe2 and intrinsic trap states in WSe2. Measurements in different FET device geometries show the multifunctionality of 2D lateral heterostructure phototransistors for efficient tuning and electrical manipulation of excitonic characteristics. Our findings pave the way for developing practical exciton-based transistors, sensors, multimodal optoelectronic and quantum technologies
format Preprint
id arxiv_https___arxiv_org_abs_2411_01257
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Trion Engineered Multimodal Transistors in Two dimensional Bilayer Semiconductor Lateral Heterostructures
Kundu, Baisali
Chakrabarty, Poulomi
Dhara, Avijit
Rosati, Roberto
Samanta, Chandan
Chakraborty, Suman K.
Sahoo, Srilagna
Dhara, Sajal
Dash, Saroj P.
Malic, Ermin
Lodha, Saurabh
Sahoo, Prasana K.
Applied Physics
Mesoscale and Nanoscale Physics
Multimodal device operations are essential to advancing the integration of 2D semiconductors in electronics, photonics, information and quantum technology. Precise control over carrier dynamics, particularly exciton generation and transport, is crucial for finetuning the functionality of optoelectronic devices based on 2D semiconductor heterostructure. However, the traditional exciton engineering methods in 2D semiconductors are mainly restricted to the artificially assembled vertical pn heterostructures with electrical or strain induced confinements. In this study, we utilized bilayer 2D lateral npn multijunction heterostructures with intrinsically spatially separated energy landscapes to achieve preferential exciton generation and manipulation without external confinement. In lateral npn FET geometry, we uncover unique and nontrivial properties, including dynamic tuning of channel photoresponsivity from positive to negative. The multimodal operation of these 2D FETs is achieved by carefully adjusting electrical bias and the impinging photon energy, enabling precise control over the trions generation and transport. Cryogenic photoluminescence measurement revealed the presence of trions in bilayer MoSe2 and intrinsic trap states in WSe2. Measurements in different FET device geometries show the multifunctionality of 2D lateral heterostructure phototransistors for efficient tuning and electrical manipulation of excitonic characteristics. Our findings pave the way for developing practical exciton-based transistors, sensors, multimodal optoelectronic and quantum technologies
title Trion Engineered Multimodal Transistors in Two dimensional Bilayer Semiconductor Lateral Heterostructures
topic Applied Physics
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2411.01257