Defects in graphite engineered by ion implantation for the self-assembly of gold nanoparticles

Fuente: arXiv
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Autori principali: Liu, Yumeng, Deng, Yanhao, Wang, Yizhuo, Wang, Li, Liu, Tong, Wei, Wei, Gong, Zhongmiao, Fan, Zhengfang, Su, Zhijuan, Wang, Yanming, Dan, Yaping
Natura: Preprint
Pubblicazione: 2024
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author Liu, Yumeng
Deng, Yanhao
Wang, Yizhuo
Wang, Li
Liu, Tong
Wei, Wei
Gong, Zhongmiao
Fan, Zhengfang
Su, Zhijuan
Wang, Yanming
Dan, Yaping
author_facet Liu, Yumeng
Deng, Yanhao
Wang, Yizhuo
Wang, Li
Liu, Tong
Wei, Wei
Gong, Zhongmiao
Fan, Zhengfang
Su, Zhijuan
Wang, Yanming
Dan, Yaping
contents Defect engineering in two-dimensional (2D) materials is essential for advancing applications such as gas sensing, single-atom catalysis, and guided nanoparticle self-assembly, enabling the creation of materials with tailored functionalities. This study investigates ion implantation effects on highly ordered pyrolytic graphite (HOPG) surfaces, using scanning tunneling microscopy (STM) and density functional theory (DFT) simulations to identify distinct defect structures. High-energy heavy ions cause inelastic scattering, increasing surface damage, while gold atoms deposited onto defect sites preferentially form atomic clusters. Through focused ion beam techniques, spatially distributed defects were engineered, guiding the self-assembly of nanoparticles. This research highlights the precision of ion irradiation for modifying HOPG surfaces, with significant implications for catalysis, nanotechnology, and the development of functional materials with controlled nanoscale properties.
format Preprint
id arxiv_https___arxiv_org_abs_2411_02204
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Defects in graphite engineered by ion implantation for the self-assembly of gold nanoparticles
Liu, Yumeng
Deng, Yanhao
Wang, Yizhuo
Wang, Li
Liu, Tong
Wei, Wei
Gong, Zhongmiao
Fan, Zhengfang
Su, Zhijuan
Wang, Yanming
Dan, Yaping
Materials Science
Mesoscale and Nanoscale Physics
Defect engineering in two-dimensional (2D) materials is essential for advancing applications such as gas sensing, single-atom catalysis, and guided nanoparticle self-assembly, enabling the creation of materials with tailored functionalities. This study investigates ion implantation effects on highly ordered pyrolytic graphite (HOPG) surfaces, using scanning tunneling microscopy (STM) and density functional theory (DFT) simulations to identify distinct defect structures. High-energy heavy ions cause inelastic scattering, increasing surface damage, while gold atoms deposited onto defect sites preferentially form atomic clusters. Through focused ion beam techniques, spatially distributed defects were engineered, guiding the self-assembly of nanoparticles. This research highlights the precision of ion irradiation for modifying HOPG surfaces, with significant implications for catalysis, nanotechnology, and the development of functional materials with controlled nanoscale properties.
title Defects in graphite engineered by ion implantation for the self-assembly of gold nanoparticles
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2411.02204