Gyrotropic Magnetic Effect in Black Phosphorus Irradiated with Bicircular Light

Fuente: arXiv
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Autores principales: Zhan, Fangyang, Jin, Xin, Ma, Da-Shuai, Fan, Jing, Yu, Peng, Xu, Dong-Hui, Wang, Rui
Formato: Preprint
Publicado: 2024
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author Zhan, Fangyang
Jin, Xin
Ma, Da-Shuai
Fan, Jing
Yu, Peng
Xu, Dong-Hui
Wang, Rui
author_facet Zhan, Fangyang
Jin, Xin
Ma, Da-Shuai
Fan, Jing
Yu, Peng
Xu, Dong-Hui
Wang, Rui
contents The gyrotropic magnetic effect (GME), which emerges as the low-frequency limit of natural gyrotopy, is a fundamental property of Bloch electrons on the Fermi surface in materials lacking inversion symmetry. While Weyl semimetals were among the first systems predicted to host the GME, this effect has not yet been experimentally observed in these materials. Here, we theoretically propose a robust scheme to generate a significant GME in anisotropic nodal-line semimetals using Floquet engineering with bicircular light (BCL). We show that BCL irradiation can selectively break spatial and time-reversal symmetries, inducing a topological phase transition from a nodal-line semimetal to a Weyl semimetal with a minimal number of Weyl nodes. Crucially, the Weyl nodes with opposite chirality are separated in energy, a key requirement for a non-zero GME. Using first-principles calculations combined with Floquet theory, we identify compressed black phosphorus as an ideal material platform. The intrinsic anisotropy of black phosphorus amplifies the GME, resulting in a measurable gyrotropic current that is several orders of magnitude larger than that in previously proposed systems. Our work not only provides a concrete path toward the experimental realization of GME but also opens new avenues for exploring the interplay of light, symmetry, and topology in quantum materials.
format Preprint
id arxiv_https___arxiv_org_abs_2411_02916
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Gyrotropic Magnetic Effect in Black Phosphorus Irradiated with Bicircular Light
Zhan, Fangyang
Jin, Xin
Ma, Da-Shuai
Fan, Jing
Yu, Peng
Xu, Dong-Hui
Wang, Rui
Materials Science
The gyrotropic magnetic effect (GME), which emerges as the low-frequency limit of natural gyrotopy, is a fundamental property of Bloch electrons on the Fermi surface in materials lacking inversion symmetry. While Weyl semimetals were among the first systems predicted to host the GME, this effect has not yet been experimentally observed in these materials. Here, we theoretically propose a robust scheme to generate a significant GME in anisotropic nodal-line semimetals using Floquet engineering with bicircular light (BCL). We show that BCL irradiation can selectively break spatial and time-reversal symmetries, inducing a topological phase transition from a nodal-line semimetal to a Weyl semimetal with a minimal number of Weyl nodes. Crucially, the Weyl nodes with opposite chirality are separated in energy, a key requirement for a non-zero GME. Using first-principles calculations combined with Floquet theory, we identify compressed black phosphorus as an ideal material platform. The intrinsic anisotropy of black phosphorus amplifies the GME, resulting in a measurable gyrotropic current that is several orders of magnitude larger than that in previously proposed systems. Our work not only provides a concrete path toward the experimental realization of GME but also opens new avenues for exploring the interplay of light, symmetry, and topology in quantum materials.
title Gyrotropic Magnetic Effect in Black Phosphorus Irradiated with Bicircular Light
topic Materials Science
url https://arxiv.org/abs/2411.02916