Single photon emitters in thin GaAsN nanowire tubes grown on Si

Fuente: arXiv
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Main Authors: Denis, Nadine, Dede, Didem, Nurmamytov, Timur, Cianci, Salvatore, Santangeli, Francesca, Felici, Marco, Boureau, Victor, Polimeni, Antonio, Rubini, Silvia, Morral, Anna Fontcuberta i, De Luca, Marta
Format: Preprint
Published: 2024
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author Denis, Nadine
Dede, Didem
Nurmamytov, Timur
Cianci, Salvatore
Santangeli, Francesca
Felici, Marco
Boureau, Victor
Polimeni, Antonio
Rubini, Silvia
Morral, Anna Fontcuberta i
De Luca, Marta
author_facet Denis, Nadine
Dede, Didem
Nurmamytov, Timur
Cianci, Salvatore
Santangeli, Francesca
Felici, Marco
Boureau, Victor
Polimeni, Antonio
Rubini, Silvia
Morral, Anna Fontcuberta i
De Luca, Marta
contents III-V nanowire heterostructures can act as sources of single and entangled photons and are enabling technologies for on-chip applications in future quantum photonic devices. The unique geometry of nanowires allows to integrate lattice-mismatched components beyond the limits of planar epilayers and to create radially and axially confined quantum structures. Here, we report the plasma-assisted molecular beam epitaxy growth of thin GaAs/GaAsN/GaAs core-multishell nanowires monolithically integrated on Si (111) substrates, overcoming the challenges caused by the low solubility of N and a high lattice mismatch. The nanowires have a GaAsN shell of 10 nm containing 2.7% N, which reduces the GaAs bandgap drastically by 400 meV. They have a symmetric core-shell structure with sharp boundaries and a defect-free zincblende phase. The high structural quality reflects in their excellent opto-electroinic properties, including remarkable single photon emission from quantum confined states in the thin GaAsN shell with a second-order autocorrelation function at zero time delay as low as 0.056.
format Preprint
id arxiv_https___arxiv_org_abs_2411_03185
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Single photon emitters in thin GaAsN nanowire tubes grown on Si
Denis, Nadine
Dede, Didem
Nurmamytov, Timur
Cianci, Salvatore
Santangeli, Francesca
Felici, Marco
Boureau, Victor
Polimeni, Antonio
Rubini, Silvia
Morral, Anna Fontcuberta i
De Luca, Marta
Optics
Materials Science
Quantum Physics
III-V nanowire heterostructures can act as sources of single and entangled photons and are enabling technologies for on-chip applications in future quantum photonic devices. The unique geometry of nanowires allows to integrate lattice-mismatched components beyond the limits of planar epilayers and to create radially and axially confined quantum structures. Here, we report the plasma-assisted molecular beam epitaxy growth of thin GaAs/GaAsN/GaAs core-multishell nanowires monolithically integrated on Si (111) substrates, overcoming the challenges caused by the low solubility of N and a high lattice mismatch. The nanowires have a GaAsN shell of 10 nm containing 2.7% N, which reduces the GaAs bandgap drastically by 400 meV. They have a symmetric core-shell structure with sharp boundaries and a defect-free zincblende phase. The high structural quality reflects in their excellent opto-electroinic properties, including remarkable single photon emission from quantum confined states in the thin GaAsN shell with a second-order autocorrelation function at zero time delay as low as 0.056.
title Single photon emitters in thin GaAsN nanowire tubes grown on Si
topic Optics
Materials Science
Quantum Physics
url https://arxiv.org/abs/2411.03185