Quantum emitters in bilayer hexagonal boron nitride

Fuente: arXiv
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Autori principali: Mehta, Reyhan, Kumar, Anshuman
Natura: Preprint
Pubblicazione: 2024
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author Mehta, Reyhan
Kumar, Anshuman
author_facet Mehta, Reyhan
Kumar, Anshuman
contents Hexagonal boron nitride (hBN) has been experimentally shown to exhibit room-temperature single-photon emission. This emission is attributed to defect states in the wide band-gap of hBN, which allow new optical transitions between these dispersion-less defect levels. In this work, we study the new spectral features introduced by interacting atomic defects in consecutive layers of bilayer hBN. Density Functional theory simulations have been carried out to calculate the energy band structure, frequency-dependent complex dielectric functions, and Kohn-Sham states to demonstrate and understand the cause of the emission enhancements. We found that placing colour centres in the vicinity of each other in bilayer hBN introduces new polarization dependent spectral features, with strong dependence on the distance and relative orientation between atomic defects. Our results provide a pathway to engineering single photon emission in hBN via inter-defect interaction.
format Preprint
id arxiv_https___arxiv_org_abs_2411_09346
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Quantum emitters in bilayer hexagonal boron nitride
Mehta, Reyhan
Kumar, Anshuman
Materials Science
Mesoscale and Nanoscale Physics
Optics
Hexagonal boron nitride (hBN) has been experimentally shown to exhibit room-temperature single-photon emission. This emission is attributed to defect states in the wide band-gap of hBN, which allow new optical transitions between these dispersion-less defect levels. In this work, we study the new spectral features introduced by interacting atomic defects in consecutive layers of bilayer hBN. Density Functional theory simulations have been carried out to calculate the energy band structure, frequency-dependent complex dielectric functions, and Kohn-Sham states to demonstrate and understand the cause of the emission enhancements. We found that placing colour centres in the vicinity of each other in bilayer hBN introduces new polarization dependent spectral features, with strong dependence on the distance and relative orientation between atomic defects. Our results provide a pathway to engineering single photon emission in hBN via inter-defect interaction.
title Quantum emitters in bilayer hexagonal boron nitride
topic Materials Science
Mesoscale and Nanoscale Physics
Optics
url https://arxiv.org/abs/2411.09346