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Bibliographic Details
Main Authors: Reinold, Anneke, Berger, Lucas, Raczkowski, Marcin, Zhao, Zhiying, Kohama, Yoshimitsu, Gen, Masaki, Gorbunov, Denis I., Skourski, Yurii, Zherlitsyn, Sergei, Assaad, Fakher F., Lorenz, Thomas, Wang, Zhe
Format: Preprint
Published: 2024
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Online Access:https://arxiv.org/abs/2411.09541
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Table of Contents:
  • We report on a comprehensive thermodynamic study of a quasi-two-dimensional (quasi-2D) quantum magnet Cu$_2$(OH)$_3$Br which in the 2D layer can be viewed as strongly coupled alternating antiferromagnetic and ferromagnetic chains. In an applied magnetic field transverse to the ordered spins below $T_N=9.3$ K, a field-induced phase transition from the 3D ordered to a disordered phase occurs at $B_c=16.3$ T for the lowest temperature, which is featured by an onset of a one-half plateau-like magnetization. By performing quantum Monte Carlo simulations of the relevant 2D model, we find that the plateau-like magnetization corresponds to a partial symmetry restoration and the full polarization in the ferromagnetic chains. Our numerical simulations also show that the magnetization saturation occurs with full symmetry restoration at a much higher field of $B_s \simeq 95$ T, corresponding to a 1D quantum phase transition in the antiferromagnetic chains. We argue that the experimentally observed field-induced phase transition at $B_c$ follows from the partial symmetry restoration and the concomitant dimensional reduction.