Three-dimensional nature of anomalous Hall conductivity in YMn6Sn6-xGax, x ~ 0.55

Fuente: arXiv
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Autores principales: Bhandari, Hari, Ning, Zhenhua, Chang, Po-Hao, Siegfried, Peter E., Regmi, Resham B., Gazzah, Mohamed El., Davydov, Albert V., Oliver, Allen G., Ke, Liqin, Mazin, Igor I., Ghimire, Nirmal J.
Formato: Preprint
Publicado: 2024
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author Bhandari, Hari
Ning, Zhenhua
Chang, Po-Hao
Siegfried, Peter E.
Regmi, Resham B.
Gazzah, Mohamed El.
Davydov, Albert V.
Oliver, Allen G.
Ke, Liqin
Mazin, Igor I.
Ghimire, Nirmal J.
author_facet Bhandari, Hari
Ning, Zhenhua
Chang, Po-Hao
Siegfried, Peter E.
Regmi, Resham B.
Gazzah, Mohamed El.
Davydov, Albert V.
Oliver, Allen G.
Ke, Liqin
Mazin, Igor I.
Ghimire, Nirmal J.
contents The unique connectivity of kagome lattices gives rise to topological properties, such as flat bands and Dirac cones. When combined with ferromagnetism and a chemical potential near the 2D Dirac points, this structure offers the potential to realize the highly sought-after topological Chern magnetotransport. Recently, there was considerable excitement surrounding this possibility in the ferrimagnetic kagome metal TbMn$_\mathbf{6}$Sn$_\mathbf{6}$. However, density functional theory (DFT) calculations reveal that the 2D Chern gap lies well above the Fermi energy, challenging its relevance in the observed anomalous Hall conductivity. Here, we investigate YMn$_\mathbf{6}$Sn$_\mathbf{5.45}$Ga$_\mathbf{0.55}$, a compound with similar crystallographic, magnetic, and electronic properties to TbMn$_\mathbf{6}$Sn$_\mathbf{6}$. Our findings show that the intrinsic anomalous Hall conductivity in this material, while comparable in magnitude to that in TbMn$_\mathbf{6}$Sn$_\mathbf{6}$, is fully three-dimensional, thus providing experimental evidence that Hall conductivity in this class of materials does not originate from 2D Chern gaps. Additionally, we confirm that the newly proposed empirical scaling relation for extrinsic Hall conductivity is universally governed by spin fluctuations.
format Preprint
id arxiv_https___arxiv_org_abs_2411_12134
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Three-dimensional nature of anomalous Hall conductivity in YMn6Sn6-xGax, x ~ 0.55
Bhandari, Hari
Ning, Zhenhua
Chang, Po-Hao
Siegfried, Peter E.
Regmi, Resham B.
Gazzah, Mohamed El.
Davydov, Albert V.
Oliver, Allen G.
Ke, Liqin
Mazin, Igor I.
Ghimire, Nirmal J.
Materials Science
The unique connectivity of kagome lattices gives rise to topological properties, such as flat bands and Dirac cones. When combined with ferromagnetism and a chemical potential near the 2D Dirac points, this structure offers the potential to realize the highly sought-after topological Chern magnetotransport. Recently, there was considerable excitement surrounding this possibility in the ferrimagnetic kagome metal TbMn$_\mathbf{6}$Sn$_\mathbf{6}$. However, density functional theory (DFT) calculations reveal that the 2D Chern gap lies well above the Fermi energy, challenging its relevance in the observed anomalous Hall conductivity. Here, we investigate YMn$_\mathbf{6}$Sn$_\mathbf{5.45}$Ga$_\mathbf{0.55}$, a compound with similar crystallographic, magnetic, and electronic properties to TbMn$_\mathbf{6}$Sn$_\mathbf{6}$. Our findings show that the intrinsic anomalous Hall conductivity in this material, while comparable in magnitude to that in TbMn$_\mathbf{6}$Sn$_\mathbf{6}$, is fully three-dimensional, thus providing experimental evidence that Hall conductivity in this class of materials does not originate from 2D Chern gaps. Additionally, we confirm that the newly proposed empirical scaling relation for extrinsic Hall conductivity is universally governed by spin fluctuations.
title Three-dimensional nature of anomalous Hall conductivity in YMn6Sn6-xGax, x ~ 0.55
topic Materials Science
url https://arxiv.org/abs/2411.12134