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Auteurs principaux: Gong, Weiyi, Sun, Tao, Bai, Hexin, Tsai, Jeng-Yuan, Ling, Haibin, Yan, Qimin
Format: Preprint
Publié: 2024
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Accès en ligne:https://arxiv.org/abs/2411.16483
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author Gong, Weiyi
Sun, Tao
Bai, Hexin
Tsai, Jeng-Yuan
Ling, Haibin
Yan, Qimin
author_facet Gong, Weiyi
Sun, Tao
Bai, Hexin
Tsai, Jeng-Yuan
Ling, Haibin
Yan, Qimin
contents Predicting electronic band structures from crystal structures is crucial for understanding structure-property correlations in materials science. First-principles approaches are accurate but computationally intensive. Recent years, machine learning (ML) has been extensively applied to this field, while existing ML models predominantly focus on band gap predictions or indirect band structure estimation via solving predicted Hamiltonians. An end-to-end model to predict band structure accurately and efficiently is still lacking. Here, we introduce a graph Transformer-based end-to-end approach that directly predicts band structures from crystal structures with high accuracy. Our method leverages the continuity of the k-path and treat continuous bands as a sequence. We demonstrate that our model not only provides accurate band structure predictions but also can derive other properties (such as band gap, band center, and band dispersion) with high accuracy. We verify the model performance on large and diverse datasets.
format Preprint
id arxiv_https___arxiv_org_abs_2411_16483
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Graph Transformer Networks for Accurate Band Structure Prediction: An End-to-End Approach
Gong, Weiyi
Sun, Tao
Bai, Hexin
Tsai, Jeng-Yuan
Ling, Haibin
Yan, Qimin
Materials Science
Machine Learning
Predicting electronic band structures from crystal structures is crucial for understanding structure-property correlations in materials science. First-principles approaches are accurate but computationally intensive. Recent years, machine learning (ML) has been extensively applied to this field, while existing ML models predominantly focus on band gap predictions or indirect band structure estimation via solving predicted Hamiltonians. An end-to-end model to predict band structure accurately and efficiently is still lacking. Here, we introduce a graph Transformer-based end-to-end approach that directly predicts band structures from crystal structures with high accuracy. Our method leverages the continuity of the k-path and treat continuous bands as a sequence. We demonstrate that our model not only provides accurate band structure predictions but also can derive other properties (such as band gap, band center, and band dispersion) with high accuracy. We verify the model performance on large and diverse datasets.
title Graph Transformer Networks for Accurate Band Structure Prediction: An End-to-End Approach
topic Materials Science
Machine Learning
url https://arxiv.org/abs/2411.16483