Analysis of a Poisson-Nernst-Planck cross-diffusion system with steric effects

Fuente: arXiv
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Main Authors: Hirvonen, Peter, Jüngel, Ansgar
Format: Preprint
Published: 2024
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_version_ 1866910716771958784
author Hirvonen, Peter
Jüngel, Ansgar
author_facet Hirvonen, Peter
Jüngel, Ansgar
contents A transient Poisson-Nernst-Planck system with steric effects is analyzed in a bounded domain with no-flux boundary conditions for the ion concentrations and mixed Dirichlet-Neumann boundary conditions for the electric potential. The steric repulsion of ions is modeled by a localized Lennard-Jones force, leading to cross-diffusion terms. The existence of global weak solutions, a weak--strong uniqueness property, and, in case of pure Neumann conditions, the exponential decay towards the thermal equilibrium state is proved. The main difficulties are the cross-diffusion terms and the different boundary conditions satisfied by the unknowns. These issues are overcome by exploiting the entropy structure of the equations and carefully taking into account the electric potential term. A numerical experiment illustrates the long-time behavior of the solutions when the potential satisfies mixed boundary conditions.
format Preprint
id arxiv_https___arxiv_org_abs_2411_17399
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Analysis of a Poisson-Nernst-Planck cross-diffusion system with steric effects
Hirvonen, Peter
Jüngel, Ansgar
Analysis of PDEs
35K51, 35A02, 35B40, 35Q92
A transient Poisson-Nernst-Planck system with steric effects is analyzed in a bounded domain with no-flux boundary conditions for the ion concentrations and mixed Dirichlet-Neumann boundary conditions for the electric potential. The steric repulsion of ions is modeled by a localized Lennard-Jones force, leading to cross-diffusion terms. The existence of global weak solutions, a weak--strong uniqueness property, and, in case of pure Neumann conditions, the exponential decay towards the thermal equilibrium state is proved. The main difficulties are the cross-diffusion terms and the different boundary conditions satisfied by the unknowns. These issues are overcome by exploiting the entropy structure of the equations and carefully taking into account the electric potential term. A numerical experiment illustrates the long-time behavior of the solutions when the potential satisfies mixed boundary conditions.
title Analysis of a Poisson-Nernst-Planck cross-diffusion system with steric effects
topic Analysis of PDEs
35K51, 35A02, 35B40, 35Q92
url https://arxiv.org/abs/2411.17399