All-passive upconversion of incoherent near-infrared light at intensities down to 10$^{-7}$ W/cm$^2$

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Hauptverfasser: Hamid, Rabeeya, Feng, Demeng, Narayanan, Pournima, Edwards, Justin S., Hu, Manchen, Belliveau, Emma, Kim, Minjeong, Deshpande, Sanket, Wan, Chenghao, Pucurimay, Linda, Czaplewski, David A., Congreve, Daniel N., Kats, Mikhail A.
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Veröffentlicht: 2024
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author Hamid, Rabeeya
Feng, Demeng
Narayanan, Pournima
Edwards, Justin S.
Hu, Manchen
Belliveau, Emma
Kim, Minjeong
Deshpande, Sanket
Wan, Chenghao
Pucurimay, Linda
Czaplewski, David A.
Congreve, Daniel N.
Kats, Mikhail A.
author_facet Hamid, Rabeeya
Feng, Demeng
Narayanan, Pournima
Edwards, Justin S.
Hu, Manchen
Belliveau, Emma
Kim, Minjeong
Deshpande, Sanket
Wan, Chenghao
Pucurimay, Linda
Czaplewski, David A.
Congreve, Daniel N.
Kats, Mikhail A.
contents Frequency upconversion, which converts low-energy photons into higher-energy ones, typically requires intense coherent illumination to drive nonlinear processes or the use of externally driven optoelectronic devices. Here, we demonstrate an upconversion system that converts low-intensity (down to ~10-7 W/cm$^2$) incoherent near-infrared (NIR) light into the visible, reaching intensities perceptible by the human eye, without the use of any external power input. Our upconverting element is enabled by the following ingredients: (1) photon upconversion via triplet-triplet annihilation in a bulk heterojunction of the organic semiconductors Y6 and rubrene; (2) plasmonic enhancement of absorption and field intensity in the heterojunction layer; (3) collection enhancement using a dichroic thin-film assembly. To enable high-resolution imaging, the upconverting element is inserted at an intermediate image plane of a dual-wavelength telescope system, which preserves the relative directionality of rays between the incident NIR light and output visible light. Our all-passive upconversion imaging system will enable NIR imaging and sensing in low-light environments under energy constraints.
format Preprint
id arxiv_https___arxiv_org_abs_2411_18707
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle All-passive upconversion of incoherent near-infrared light at intensities down to 10$^{-7}$ W/cm$^2$
Hamid, Rabeeya
Feng, Demeng
Narayanan, Pournima
Edwards, Justin S.
Hu, Manchen
Belliveau, Emma
Kim, Minjeong
Deshpande, Sanket
Wan, Chenghao
Pucurimay, Linda
Czaplewski, David A.
Congreve, Daniel N.
Kats, Mikhail A.
Optics
Mesoscale and Nanoscale Physics
Materials Science
Applied Physics
Frequency upconversion, which converts low-energy photons into higher-energy ones, typically requires intense coherent illumination to drive nonlinear processes or the use of externally driven optoelectronic devices. Here, we demonstrate an upconversion system that converts low-intensity (down to ~10-7 W/cm$^2$) incoherent near-infrared (NIR) light into the visible, reaching intensities perceptible by the human eye, without the use of any external power input. Our upconverting element is enabled by the following ingredients: (1) photon upconversion via triplet-triplet annihilation in a bulk heterojunction of the organic semiconductors Y6 and rubrene; (2) plasmonic enhancement of absorption and field intensity in the heterojunction layer; (3) collection enhancement using a dichroic thin-film assembly. To enable high-resolution imaging, the upconverting element is inserted at an intermediate image plane of a dual-wavelength telescope system, which preserves the relative directionality of rays between the incident NIR light and output visible light. Our all-passive upconversion imaging system will enable NIR imaging and sensing in low-light environments under energy constraints.
title All-passive upconversion of incoherent near-infrared light at intensities down to 10$^{-7}$ W/cm$^2$
topic Optics
Mesoscale and Nanoscale Physics
Materials Science
Applied Physics
url https://arxiv.org/abs/2411.18707