Impact of Thermal Effects on the Current-Tunable Electrical Transport in the Ferrimagnetic Semiconductor Mn$_3$Si$_2$Te$_6$

Fuente: arXiv
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Main Authors: Zhang, Yiyue, Jin, Xin, Li, ZeYu, Yang, Kunya, Wei, Linlin, Mi, Xinrun, Wang, Aifeng, Zhou, Xiaoyuan, Yang, Xiaolong, Chai, Yisheng, He, Mingquan
Format: Preprint
Published: 2024
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author Zhang, Yiyue
Jin, Xin
Li, ZeYu
Yang, Kunya
Wei, Linlin
Mi, Xinrun
Wang, Aifeng
Zhou, Xiaoyuan
Yang, Xiaolong
Chai, Yisheng
He, Mingquan
author_facet Zhang, Yiyue
Jin, Xin
Li, ZeYu
Yang, Kunya
Wei, Linlin
Mi, Xinrun
Wang, Aifeng
Zhou, Xiaoyuan
Yang, Xiaolong
Chai, Yisheng
He, Mingquan
contents In the ferrimagnetic semiconductor Mn$_3$Si$_2$Te$_6$, a colossal magnetoresistance (CMR) is observed only when a magnetic field is applied along the magnetic hard axis ($\mathbf{H}\parallel c$). This phenomenon suggests an unconventional CMR mechanism potentially driven by the interplay between magnetism, topological band structure, and/or chiral orbital currents (COC). By comparing electrical resistance measurements using continuous direct currents and pulse currents, we found that the current-induced insulator-metal transition, supporting the COC-driven CMR mechanism, is likely a consequence of Joule heating effects. First-principles calculations reveal a pronounced band gap reduction upon tilting the magnetic moments toward the $c$-axis, accompanied by increased carrier concentration and Fermi velocity. Combining spin orientation-dependent electronic structure with Boltzmann transport theory, the calculated electrical resistance closely reproduces the CMR observed experimentally. These findings suggest that the CMR in Mn$_3$Si$_2$Te$_6$ stems primarily from band gap reduction induced by partial polarization of magnetic moments along the magnetic hard axis.
format Preprint
id arxiv_https___arxiv_org_abs_2412_01518
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Impact of Thermal Effects on the Current-Tunable Electrical Transport in the Ferrimagnetic Semiconductor Mn$_3$Si$_2$Te$_6$
Zhang, Yiyue
Jin, Xin
Li, ZeYu
Yang, Kunya
Wei, Linlin
Mi, Xinrun
Wang, Aifeng
Zhou, Xiaoyuan
Yang, Xiaolong
Chai, Yisheng
He, Mingquan
Materials Science
Strongly Correlated Electrons
In the ferrimagnetic semiconductor Mn$_3$Si$_2$Te$_6$, a colossal magnetoresistance (CMR) is observed only when a magnetic field is applied along the magnetic hard axis ($\mathbf{H}\parallel c$). This phenomenon suggests an unconventional CMR mechanism potentially driven by the interplay between magnetism, topological band structure, and/or chiral orbital currents (COC). By comparing electrical resistance measurements using continuous direct currents and pulse currents, we found that the current-induced insulator-metal transition, supporting the COC-driven CMR mechanism, is likely a consequence of Joule heating effects. First-principles calculations reveal a pronounced band gap reduction upon tilting the magnetic moments toward the $c$-axis, accompanied by increased carrier concentration and Fermi velocity. Combining spin orientation-dependent electronic structure with Boltzmann transport theory, the calculated electrical resistance closely reproduces the CMR observed experimentally. These findings suggest that the CMR in Mn$_3$Si$_2$Te$_6$ stems primarily from band gap reduction induced by partial polarization of magnetic moments along the magnetic hard axis.
title Impact of Thermal Effects on the Current-Tunable Electrical Transport in the Ferrimagnetic Semiconductor Mn$_3$Si$_2$Te$_6$
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2412.01518