Double-edged Role of Interactions in Superconducting Twisted Bilayer Graphene

Fuente: arXiv
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Main Authors: Gao, Xueshi, Jimeno-Pozo, Alejandro, Pantaleon, Pierre A., Codecido, Emilio, Sharifi, Daria L., Zhang, Zheneng, Liu, Youwei, Watanabe, Kenji, Taniguchi, Takashi, Bockrath, Marc W., Guinea, Francisco, Lau, Chun Ning
Format: Preprint
Published: 2024
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author Gao, Xueshi
Jimeno-Pozo, Alejandro
Pantaleon, Pierre A.
Codecido, Emilio
Sharifi, Daria L.
Zhang, Zheneng
Liu, Youwei
Watanabe, Kenji
Taniguchi, Takashi
Bockrath, Marc W.
Guinea, Francisco
Lau, Chun Ning
author_facet Gao, Xueshi
Jimeno-Pozo, Alejandro
Pantaleon, Pierre A.
Codecido, Emilio
Sharifi, Daria L.
Zhang, Zheneng
Liu, Youwei
Watanabe, Kenji
Taniguchi, Takashi
Bockrath, Marc W.
Guinea, Francisco
Lau, Chun Ning
contents For the unconventional superconducting phases in moire materials, a critical question is the role played by electronic interactions in the formation of Cooper pairs. In twisted bilayer graphene (tBLG), the strength of electronic interactions can be reduced by increasing the twist angle or screening provided by the dielectric medium. In this work, we place tBLG at 3-4 nm above bulk SrTiO3 substrates, which have a large yet tunable dielectric constant. By raising the dielectric constant in situ in a magic angle device, we observe suppression of both the height and the width of the entire superconducting dome, thus demonstrating that, unlike conventional superconductors, the pairing mechanism in tBLG is strongly dependent on electronic interactions. Interestingly, in contrast to the absence of superconductivity in devices on SiO2 with angle>1.3 deg, we observe a superconducting pocket in a large-angle (angle=1.4 deg) tBLG/STO device while the correlated insulating states are absent. These experimental results are in qualitative agreement with a theoretical model in which the pairing mechanism arises from Coulomb interactions that are screened by plasmons, electron-hole pairs, and longitudinal acoustic phonons. Our results highlight the unconventional nature of the superconductivity in tBLG, the double-edged role played by electronic interactions in its formation, as well as their complex interplay with the correlated insulating states.
format Preprint
id arxiv_https___arxiv_org_abs_2412_01578
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Double-edged Role of Interactions in Superconducting Twisted Bilayer Graphene
Gao, Xueshi
Jimeno-Pozo, Alejandro
Pantaleon, Pierre A.
Codecido, Emilio
Sharifi, Daria L.
Zhang, Zheneng
Liu, Youwei
Watanabe, Kenji
Taniguchi, Takashi
Bockrath, Marc W.
Guinea, Francisco
Lau, Chun Ning
Mesoscale and Nanoscale Physics
Superconductivity
For the unconventional superconducting phases in moire materials, a critical question is the role played by electronic interactions in the formation of Cooper pairs. In twisted bilayer graphene (tBLG), the strength of electronic interactions can be reduced by increasing the twist angle or screening provided by the dielectric medium. In this work, we place tBLG at 3-4 nm above bulk SrTiO3 substrates, which have a large yet tunable dielectric constant. By raising the dielectric constant in situ in a magic angle device, we observe suppression of both the height and the width of the entire superconducting dome, thus demonstrating that, unlike conventional superconductors, the pairing mechanism in tBLG is strongly dependent on electronic interactions. Interestingly, in contrast to the absence of superconductivity in devices on SiO2 with angle>1.3 deg, we observe a superconducting pocket in a large-angle (angle=1.4 deg) tBLG/STO device while the correlated insulating states are absent. These experimental results are in qualitative agreement with a theoretical model in which the pairing mechanism arises from Coulomb interactions that are screened by plasmons, electron-hole pairs, and longitudinal acoustic phonons. Our results highlight the unconventional nature of the superconductivity in tBLG, the double-edged role played by electronic interactions in its formation, as well as their complex interplay with the correlated insulating states.
title Double-edged Role of Interactions in Superconducting Twisted Bilayer Graphene
topic Mesoscale and Nanoscale Physics
Superconductivity
url https://arxiv.org/abs/2412.01578