Terahertz stimulated parametric downconversion of a magnon mode in an antiferromagnet

Fuente: arXiv
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Main Authors: Zhang, Zhuquan, Chien, Yu-Che, Wong, Man Tou, Gao, Frank Y., Liu, Zi-Jie, Ma, Xiaoxuan, Cao, Shixun, Baldini, Edoardo, Nelson, Keith A.
Format: Preprint
Published: 2024
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author Zhang, Zhuquan
Chien, Yu-Che
Wong, Man Tou
Gao, Frank Y.
Liu, Zi-Jie
Ma, Xiaoxuan
Cao, Shixun
Baldini, Edoardo
Nelson, Keith A.
author_facet Zhang, Zhuquan
Chien, Yu-Che
Wong, Man Tou
Gao, Frank Y.
Liu, Zi-Jie
Ma, Xiaoxuan
Cao, Shixun
Baldini, Edoardo
Nelson, Keith A.
contents In condensed matter systems, interactions between collective modes offer avenues for nonlinear coherent manipulation of coupled excitations and quantum phases. Antiferromagnets, with their inherently coupled magnon modes, provide a promising platform for nonlinear control of microscopic spin waves and macroscopic magnetization. However, nonlinear magnon-magnon interactions have been only partially elaborated, leaving key gaps in the prospects for potential ultrahigh-bandwidth magnonic signal processing. Here, we use a pair of intense terahertz pulses to sequentially excite two distinct coherent magnon modes in an antiferromagnet and find that the magnon mode with a lower frequency undergoes amplification when the higher-frequency mode is driven. We unveil the nonlinear excitation pathways of this stimulated parametric downconversion process by using polarization-selective two-dimensional terahertz spectroscopy. Our work provides fundamental insights into nonlinear magnonics in antiferromagnets, laying the groundwork for forthcoming spintronic and magnonic devices based on nonlinear magnon-magnon interactions.
format Preprint
id arxiv_https___arxiv_org_abs_2412_01989
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Terahertz stimulated parametric downconversion of a magnon mode in an antiferromagnet
Zhang, Zhuquan
Chien, Yu-Che
Wong, Man Tou
Gao, Frank Y.
Liu, Zi-Jie
Ma, Xiaoxuan
Cao, Shixun
Baldini, Edoardo
Nelson, Keith A.
Materials Science
In condensed matter systems, interactions between collective modes offer avenues for nonlinear coherent manipulation of coupled excitations and quantum phases. Antiferromagnets, with their inherently coupled magnon modes, provide a promising platform for nonlinear control of microscopic spin waves and macroscopic magnetization. However, nonlinear magnon-magnon interactions have been only partially elaborated, leaving key gaps in the prospects for potential ultrahigh-bandwidth magnonic signal processing. Here, we use a pair of intense terahertz pulses to sequentially excite two distinct coherent magnon modes in an antiferromagnet and find that the magnon mode with a lower frequency undergoes amplification when the higher-frequency mode is driven. We unveil the nonlinear excitation pathways of this stimulated parametric downconversion process by using polarization-selective two-dimensional terahertz spectroscopy. Our work provides fundamental insights into nonlinear magnonics in antiferromagnets, laying the groundwork for forthcoming spintronic and magnonic devices based on nonlinear magnon-magnon interactions.
title Terahertz stimulated parametric downconversion of a magnon mode in an antiferromagnet
topic Materials Science
url https://arxiv.org/abs/2412.01989