Evidence of spin reorientation transition below 150 K from magnetic force microscopy in a ferromagnetic BiFeO$_3$ thin film

Fuente: arXiv
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Main Authors: Goswami, Sudipta, Mishra, Shubhankar, Sahoo, Kishor Kumar, Brajesh, Kumar, Sahoo, Mihir Ranjan, Chatterjee, Subhashree, Mukherjee, Devajyoti, Pradhan, Kalpataru, Garg, Ashish, Ghosh, Chandan Kumar, Bhattacharya, Dipten
Format: Preprint
Published: 2024
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author Goswami, Sudipta
Mishra, Shubhankar
Sahoo, Kishor Kumar
Brajesh, Kumar
Sahoo, Mihir Ranjan
Chatterjee, Subhashree
Mukherjee, Devajyoti
Pradhan, Kalpataru
Garg, Ashish
Ghosh, Chandan Kumar
Bhattacharya, Dipten
author_facet Goswami, Sudipta
Mishra, Shubhankar
Sahoo, Kishor Kumar
Brajesh, Kumar
Sahoo, Mihir Ranjan
Chatterjee, Subhashree
Mukherjee, Devajyoti
Pradhan, Kalpataru
Garg, Ashish
Ghosh, Chandan Kumar
Bhattacharya, Dipten
contents We investigated the magnetic transitions in BiFeO$_3$ at low temperature (5-300 K) and observed nearly 90$^o$ rotation of magnetic domains (imaged by vertical magnetic force microscopy) across 150 K in an epitaxial thin film of thickness $\sim$36 nm. It offers a clear evidence of spin reorientation transition. It also corroborates the transition observed below $\sim$150 K in the zero-field-cooled and field-cooled magnetization versus temperature data. The field-driven 180$^o$ domain switching at room temperature, on the other hand, signifies presence of ferromagnetism. Since bulk antiferromagnetic BiFeO$_3$ does not exhibit such a transition, this observation in ferromagnetic thin film of BiFeO$_3$ indicates a radical effect because of epitaxial strain. Density functional theory based first-principles calculations too reveal that combined in- and out-of-plane epitaxial strain induces magnetic transition from G- to C-type structure in BiFeO$_3$.
format Preprint
id arxiv_https___arxiv_org_abs_2412_03180
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Evidence of spin reorientation transition below 150 K from magnetic force microscopy in a ferromagnetic BiFeO$_3$ thin film
Goswami, Sudipta
Mishra, Shubhankar
Sahoo, Kishor Kumar
Brajesh, Kumar
Sahoo, Mihir Ranjan
Chatterjee, Subhashree
Mukherjee, Devajyoti
Pradhan, Kalpataru
Garg, Ashish
Ghosh, Chandan Kumar
Bhattacharya, Dipten
Materials Science
Strongly Correlated Electrons
We investigated the magnetic transitions in BiFeO$_3$ at low temperature (5-300 K) and observed nearly 90$^o$ rotation of magnetic domains (imaged by vertical magnetic force microscopy) across 150 K in an epitaxial thin film of thickness $\sim$36 nm. It offers a clear evidence of spin reorientation transition. It also corroborates the transition observed below $\sim$150 K in the zero-field-cooled and field-cooled magnetization versus temperature data. The field-driven 180$^o$ domain switching at room temperature, on the other hand, signifies presence of ferromagnetism. Since bulk antiferromagnetic BiFeO$_3$ does not exhibit such a transition, this observation in ferromagnetic thin film of BiFeO$_3$ indicates a radical effect because of epitaxial strain. Density functional theory based first-principles calculations too reveal that combined in- and out-of-plane epitaxial strain induces magnetic transition from G- to C-type structure in BiFeO$_3$.
title Evidence of spin reorientation transition below 150 K from magnetic force microscopy in a ferromagnetic BiFeO$_3$ thin film
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2412.03180