Spin and Orbital Rashba effects at the Ni/HfO$_2$ interface

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Hauptverfasser: Pezo, Armando, Saul, Andrés, Manchon, Aurélien, Arras, Rémi
Format: Preprint
Veröffentlicht: 2024
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author Pezo, Armando
Saul, Andrés
Manchon, Aurélien
Arras, Rémi
author_facet Pezo, Armando
Saul, Andrés
Manchon, Aurélien
Arras, Rémi
contents We predict the giant ferroelectric control of interfacial properties of Ni/HfO2, namely, (i) the magnetocrystalline anisotropy and (ii) the inverse spin and orbital Rashba effects. The reversible control of magnetic properties using electric gating is a promising route to low-energy consumption magnetic devices, including memories and logic gates. Synthetic multiferroics, composed of a ferroelectric in proximity to a magnet, stand out as a promising platform for such devices. Using a combination of $ab$ $initio$ simulations and transport calculations, we demonstrate that reversing the electric polarization modulates the interface magnetocrystalline anisotropy from in-plane to out-of-plane. This modulation compares favorably with recent reports obtained upon electromigration induced by ionic gating. In addition, we find that the current-driven spin and orbital densities at the interface can be modulated by about 50% and 30%, respectively. This giant modulation of the spin-charge and orbit-charge conversion efficiencies opens appealing avenues for voltage-controlled spin- and orbitronics devices.
format Preprint
id arxiv_https___arxiv_org_abs_2412_04927
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Spin and Orbital Rashba effects at the Ni/HfO$_2$ interface
Pezo, Armando
Saul, Andrés
Manchon, Aurélien
Arras, Rémi
Materials Science
We predict the giant ferroelectric control of interfacial properties of Ni/HfO2, namely, (i) the magnetocrystalline anisotropy and (ii) the inverse spin and orbital Rashba effects. The reversible control of magnetic properties using electric gating is a promising route to low-energy consumption magnetic devices, including memories and logic gates. Synthetic multiferroics, composed of a ferroelectric in proximity to a magnet, stand out as a promising platform for such devices. Using a combination of $ab$ $initio$ simulations and transport calculations, we demonstrate that reversing the electric polarization modulates the interface magnetocrystalline anisotropy from in-plane to out-of-plane. This modulation compares favorably with recent reports obtained upon electromigration induced by ionic gating. In addition, we find that the current-driven spin and orbital densities at the interface can be modulated by about 50% and 30%, respectively. This giant modulation of the spin-charge and orbit-charge conversion efficiencies opens appealing avenues for voltage-controlled spin- and orbitronics devices.
title Spin and Orbital Rashba effects at the Ni/HfO$_2$ interface
topic Materials Science
url https://arxiv.org/abs/2412.04927