Interplay of Quasi-Quantum Hall Effect and Coulomb Disorder in Semimetals

Fuente: arXiv
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Autores principales: Leahy, Ian A., Rice, Anthony D., Nelson, Jocienne N., Ness, Herve, van Schilfgaarde, Mark, Graf, David, Suslov, Alexey, Pan, Wei, Alberi, Kirstin
Formato: Preprint
Publicado: 2024
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author Leahy, Ian A.
Rice, Anthony D.
Nelson, Jocienne N.
Ness, Herve
van Schilfgaarde, Mark
Graf, David
Suslov, Alexey
Pan, Wei
Alberi, Kirstin
author_facet Leahy, Ian A.
Rice, Anthony D.
Nelson, Jocienne N.
Ness, Herve
van Schilfgaarde, Mark
Graf, David
Suslov, Alexey
Pan, Wei
Alberi, Kirstin
contents Low carrier densities in topological semimetals (TSMs) enable the exploration of novel magnetotransport in the quantum limit (QL). Recent findings consistent with 3D quasi-quantum Hall effect (QQHE) have positioned TSMs as promising platforms for exploring 3D quantum Hall transport, but the lack of tunability in the Fermi level has thus far limited the ability to observe a QQHE signal. Here, we tune the defect concentrations in the Dirac semimetal Cd${}_3$As${}_2$ to achieve ultra-low carrier concentrations at 2 K around $2.9\times10^{16}$cm${}^{-3}$, giving way to QQHE signal at modest fields near 10 T. At low carrier densities, where QQHE is most accessible, we find that clear QQHE is obscured by a carrier density dependent background originating from Coulomb disorder from charged point defects and Landau level broadening. Our results highlight the interplay between QQHE and Coulomb disorder, demonstrating that clear observation of QQHE in TSMs intricately depends on Fermi level and disorder magnitudes. We find that Coulomb disorder, as theoretically predicted, is an essential ingredient for understanding the magnetoresistivity for a spectrum of Fermi levels in Cd${}_3$As${}_2$, anchoring the role of defects and charged disorder in TSM applications. We discuss future constraints and opportunities in exploring 3D QQHE and quantum Hall effects in TSMs.
format Preprint
id arxiv_https___arxiv_org_abs_2412_05273
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Interplay of Quasi-Quantum Hall Effect and Coulomb Disorder in Semimetals
Leahy, Ian A.
Rice, Anthony D.
Nelson, Jocienne N.
Ness, Herve
van Schilfgaarde, Mark
Graf, David
Suslov, Alexey
Pan, Wei
Alberi, Kirstin
Materials Science
Low carrier densities in topological semimetals (TSMs) enable the exploration of novel magnetotransport in the quantum limit (QL). Recent findings consistent with 3D quasi-quantum Hall effect (QQHE) have positioned TSMs as promising platforms for exploring 3D quantum Hall transport, but the lack of tunability in the Fermi level has thus far limited the ability to observe a QQHE signal. Here, we tune the defect concentrations in the Dirac semimetal Cd${}_3$As${}_2$ to achieve ultra-low carrier concentrations at 2 K around $2.9\times10^{16}$cm${}^{-3}$, giving way to QQHE signal at modest fields near 10 T. At low carrier densities, where QQHE is most accessible, we find that clear QQHE is obscured by a carrier density dependent background originating from Coulomb disorder from charged point defects and Landau level broadening. Our results highlight the interplay between QQHE and Coulomb disorder, demonstrating that clear observation of QQHE in TSMs intricately depends on Fermi level and disorder magnitudes. We find that Coulomb disorder, as theoretically predicted, is an essential ingredient for understanding the magnetoresistivity for a spectrum of Fermi levels in Cd${}_3$As${}_2$, anchoring the role of defects and charged disorder in TSM applications. We discuss future constraints and opportunities in exploring 3D QQHE and quantum Hall effects in TSMs.
title Interplay of Quasi-Quantum Hall Effect and Coulomb Disorder in Semimetals
topic Materials Science
url https://arxiv.org/abs/2412.05273