Tunable Orbital Thermoelectric Transport with Spin-Valley Coupling in Ferromagnetic Transition Metal Dichalcogenides

Fuente: arXiv
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Main Authors: Ji, Shilei, Yang, Jianping, Gao, Li, Li, Xing'ao
Format: Preprint
Published: 2024
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author Ji, Shilei
Yang, Jianping
Gao, Li
Li, Xing'ao
author_facet Ji, Shilei
Yang, Jianping
Gao, Li
Li, Xing'ao
contents In valleytronic devices, the valley transport of electrons can carry not only charge but also spin angular momentum (SAM) and orbital angular momentum (OAM). However, investigations on thermoelectric transport of OAM manipulated by valley degrees of freedom remain limited. Here, using the ferromagnetic transition metal dichalcogenides RuCl$_2$ as an example, we investigate valley-contrasting Berry curvature and demonstrate its role in generating valley-dependent anomalous and orbital Nernst effects. The thermoelectric transport of OAM is shown to be modulated by intrinsic spin polarization and exhibits characteristics of valley-orbital coupling. Furthermore, we show that spin-valley coupling plays a crucial role in controlling the orbital Nernst effect and distinguishing it from the anomalous Nernst effect. Based on these findings, we propose a thermoelectric transport mechanism for generating pure orbital currents.
format Preprint
id arxiv_https___arxiv_org_abs_2412_07266
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Tunable Orbital Thermoelectric Transport with Spin-Valley Coupling in Ferromagnetic Transition Metal Dichalcogenides
Ji, Shilei
Yang, Jianping
Gao, Li
Li, Xing'ao
Computational Physics
In valleytronic devices, the valley transport of electrons can carry not only charge but also spin angular momentum (SAM) and orbital angular momentum (OAM). However, investigations on thermoelectric transport of OAM manipulated by valley degrees of freedom remain limited. Here, using the ferromagnetic transition metal dichalcogenides RuCl$_2$ as an example, we investigate valley-contrasting Berry curvature and demonstrate its role in generating valley-dependent anomalous and orbital Nernst effects. The thermoelectric transport of OAM is shown to be modulated by intrinsic spin polarization and exhibits characteristics of valley-orbital coupling. Furthermore, we show that spin-valley coupling plays a crucial role in controlling the orbital Nernst effect and distinguishing it from the anomalous Nernst effect. Based on these findings, we propose a thermoelectric transport mechanism for generating pure orbital currents.
title Tunable Orbital Thermoelectric Transport with Spin-Valley Coupling in Ferromagnetic Transition Metal Dichalcogenides
topic Computational Physics
url https://arxiv.org/abs/2412.07266