Sodium diffusion in alkali feldspars: Towards the impact of Al/Si ordering

Fuente: arXiv
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Main Authors: Kulitckaya, Olga, Gorfer, Alexander, Petrishcheva, Elena, Tas, Bengü, Kulitckii, Vladislav, Wilde, Gerhard, Abart, Rainer, Divinski, Sergiy V.
Format: Preprint
Published: 2024
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author Kulitckaya, Olga
Gorfer, Alexander
Petrishcheva, Elena
Tas, Bengü
Kulitckii, Vladislav
Wilde, Gerhard
Abart, Rainer
Divinski, Sergiy V.
author_facet Kulitckaya, Olga
Gorfer, Alexander
Petrishcheva, Elena
Tas, Bengü
Kulitckii, Vladislav
Wilde, Gerhard
Abart, Rainer
Divinski, Sergiy V.
contents Tracer diffusion of Na in natural alkali feldspars including sanidine, adularia and orthoclase with different Na:K ratios is measured using the radiotracer technique and applying the 22Na radioisotope. The tracer diffusion measurements along the crystallographic directions perpendicular to (001) and (010) in alularia feldspar reveled a slight (within a factor of two to three) anisotropy of Na diffusion with the faster diffusion rates along the perpendicular to (001) directions, while this difference was less prominent in orthoclase. The anisotropy of Na diffusion is specifically addressed for orthoclase and the full diffusion tensor is determined. The impact of temperature and composition on diffusion in natural alkali feldspars is discussed with respect to impurities and intrinsic defects. The state of Al/Si ordering is proposed to have a significant influence on the Na diffusion rates in alkali feldspars.
format Preprint
id arxiv_https___arxiv_org_abs_2412_11635
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Sodium diffusion in alkali feldspars: Towards the impact of Al/Si ordering
Kulitckaya, Olga
Gorfer, Alexander
Petrishcheva, Elena
Tas, Bengü
Kulitckii, Vladislav
Wilde, Gerhard
Abart, Rainer
Divinski, Sergiy V.
Materials Science
Tracer diffusion of Na in natural alkali feldspars including sanidine, adularia and orthoclase with different Na:K ratios is measured using the radiotracer technique and applying the 22Na radioisotope. The tracer diffusion measurements along the crystallographic directions perpendicular to (001) and (010) in alularia feldspar reveled a slight (within a factor of two to three) anisotropy of Na diffusion with the faster diffusion rates along the perpendicular to (001) directions, while this difference was less prominent in orthoclase. The anisotropy of Na diffusion is specifically addressed for orthoclase and the full diffusion tensor is determined. The impact of temperature and composition on diffusion in natural alkali feldspars is discussed with respect to impurities and intrinsic defects. The state of Al/Si ordering is proposed to have a significant influence on the Na diffusion rates in alkali feldspars.
title Sodium diffusion in alkali feldspars: Towards the impact of Al/Si ordering
topic Materials Science
url https://arxiv.org/abs/2412.11635