Paradoxical creation of a polydomain pattern by electric field in BaTiO3 crystal

Fuente: arXiv
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Hauptverfasser: Bednyakov, Petr S., Yudin, Petr V., Tagantsev, Alexander K., Hlinka, Jiří
Format: Preprint
Veröffentlicht: 2024
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author Bednyakov, Petr S.
Yudin, Petr V.
Tagantsev, Alexander K.
Hlinka, Jiří
author_facet Bednyakov, Petr S.
Yudin, Petr V.
Tagantsev, Alexander K.
Hlinka, Jiří
contents It is known that ferroelectric single crystals can be turned from a polydomain to a monodomain state by the application of an electric field. Here we report an unexpected opposite effect: the formation of through-the-crystal polydomain pattern in a monodomain BaTiO3 crystal in response to the applied electric field favoring the initial orientation of the polarization. The effect is achieved for special electric field direction which equally selects two domain states, which are present in the polydomain pattern. At the formation of the pattern, the new wedge domains propagate from the sides of the sample in the direction transverse to the electric field. The observations are rationalized in terms of a simple analytical model treating energies of competing domain configurations as functions of the electric field. The results of the analytical treatment are supported by phase field modeling.
format Preprint
id arxiv_https___arxiv_org_abs_2412_13886
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Paradoxical creation of a polydomain pattern by electric field in BaTiO3 crystal
Bednyakov, Petr S.
Yudin, Petr V.
Tagantsev, Alexander K.
Hlinka, Jiří
Materials Science
It is known that ferroelectric single crystals can be turned from a polydomain to a monodomain state by the application of an electric field. Here we report an unexpected opposite effect: the formation of through-the-crystal polydomain pattern in a monodomain BaTiO3 crystal in response to the applied electric field favoring the initial orientation of the polarization. The effect is achieved for special electric field direction which equally selects two domain states, which are present in the polydomain pattern. At the formation of the pattern, the new wedge domains propagate from the sides of the sample in the direction transverse to the electric field. The observations are rationalized in terms of a simple analytical model treating energies of competing domain configurations as functions of the electric field. The results of the analytical treatment are supported by phase field modeling.
title Paradoxical creation of a polydomain pattern by electric field in BaTiO3 crystal
topic Materials Science
url https://arxiv.org/abs/2412.13886