Simultaneous achievement of record-breaking colossal magnetoresistance and angular magnetoresistance in an antiferromagnetic semiconductor EuSe2

Fuente: arXiv
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Autori principali: Dong, Qingxin, Yang, Pengtao, Liu, Zhihao, Wang, Yuzhi, Liu, Ziyi, Shi, Tong, Tian, Zhaoming, Sun, Jianping, Uwatoko, Yoshiya, Wu, Quansheng, Chen, Genfu, Wang, Bosen, Cheng, Jinguang
Natura: Preprint
Pubblicazione: 2024
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author Dong, Qingxin
Yang, Pengtao
Liu, Zhihao
Wang, Yuzhi
Liu, Ziyi
Shi, Tong
Tian, Zhaoming
Sun, Jianping
Uwatoko, Yoshiya
Wu, Quansheng
Chen, Genfu
Wang, Bosen
Cheng, Jinguang
author_facet Dong, Qingxin
Yang, Pengtao
Liu, Zhihao
Wang, Yuzhi
Liu, Ziyi
Shi, Tong
Tian, Zhaoming
Sun, Jianping
Uwatoko, Yoshiya
Wu, Quansheng
Chen, Genfu
Wang, Bosen
Cheng, Jinguang
contents Magnetoresistance effect lays the foundation for spintronics, magnetic sensors and hard drives. The pursuit of magnetic materials with colossal magnetoresistance (CMR) and/or angular magnetoresistance (AMR) has attracted enduring research interest and extensive investigations over past decades. Here we report on the discovery of field-induced record-breaking CMR of ~ -10^14 % and AMR ~ 10^14% achieved simultaneously in an antiferromagnetic rare-earth dichalcogenide EuSe2. Such intriguing observations are attributed to strong magnetic anisotropy and magnetic-field induced antiferromagnetic to ferromagnetic transition of the localized Eu2+ spins, which in turn closes the bandgap by lifting the degeneracy of Se-5p bands near Fermi level. Our DFT calculations perfectly replicate the experimental findings based on the Brillouin function and carries transport model. The present work provides a potential simple antiferromagnetic material for achieving angle-sensitive spintronic devices.
format Preprint
id arxiv_https___arxiv_org_abs_2412_17594
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Simultaneous achievement of record-breaking colossal magnetoresistance and angular magnetoresistance in an antiferromagnetic semiconductor EuSe2
Dong, Qingxin
Yang, Pengtao
Liu, Zhihao
Wang, Yuzhi
Liu, Ziyi
Shi, Tong
Tian, Zhaoming
Sun, Jianping
Uwatoko, Yoshiya
Wu, Quansheng
Chen, Genfu
Wang, Bosen
Cheng, Jinguang
Strongly Correlated Electrons
Materials Science
Magnetoresistance effect lays the foundation for spintronics, magnetic sensors and hard drives. The pursuit of magnetic materials with colossal magnetoresistance (CMR) and/or angular magnetoresistance (AMR) has attracted enduring research interest and extensive investigations over past decades. Here we report on the discovery of field-induced record-breaking CMR of ~ -10^14 % and AMR ~ 10^14% achieved simultaneously in an antiferromagnetic rare-earth dichalcogenide EuSe2. Such intriguing observations are attributed to strong magnetic anisotropy and magnetic-field induced antiferromagnetic to ferromagnetic transition of the localized Eu2+ spins, which in turn closes the bandgap by lifting the degeneracy of Se-5p bands near Fermi level. Our DFT calculations perfectly replicate the experimental findings based on the Brillouin function and carries transport model. The present work provides a potential simple antiferromagnetic material for achieving angle-sensitive spintronic devices.
title Simultaneous achievement of record-breaking colossal magnetoresistance and angular magnetoresistance in an antiferromagnetic semiconductor EuSe2
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2412.17594