Evidence for a $\mathbb{Z}_{2}$ Dirac spin liquid in the generalized Shastry-Sutherland model

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Main Authors: Maity, Atanu, Ferrari, Francesco, Capponi, Sylvain, Penc, Karlo, Potten, Janik, Müller, Tobias, Feuerpfeil, Andreas, Thomale, Ronny, Lee, Jong Yeon, Samajdar, Rhine, Iqbal, Yasir
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Published: 2024
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author Maity, Atanu
Ferrari, Francesco
Capponi, Sylvain
Penc, Karlo
Potten, Janik
Müller, Tobias
Feuerpfeil, Andreas
Thomale, Ronny
Lee, Jong Yeon
Samajdar, Rhine
Iqbal, Yasir
author_facet Maity, Atanu
Ferrari, Francesco
Capponi, Sylvain
Penc, Karlo
Potten, Janik
Müller, Tobias
Feuerpfeil, Andreas
Thomale, Ronny
Lee, Jong Yeon
Samajdar, Rhine
Iqbal, Yasir
contents We present a multimethod investigation into the nature of the recently reported quantum spin liquid (QSL) phase in the spin-$1/2$ Heisenberg antiferromagnet on the Shastry-Sutherland lattice. A comprehensive projective symmetry group classification of fermionic mean-field Ansätze on this lattice yields 46 U(1) and 80 $\mathbb{Z}_2$ states. Using density-matrix renormalization group (DMRG) and exact diagonalization calculations, we find that the Shastry-Sutherland model and the square-lattice $J_1$-$J_2$ Heisenberg antiferromagnet share the same QSL phase. Motivated by this observation, we establish an explicit mapping of our Ansätze to those on the square lattice, and identify the counterpart of the square-lattice $\mathbb{Z}_2$ Dirac QSL (Z2A$zz$13) in the Shastry-Sutherland system. Employing state-of-the-art variational Monte Carlo calculations with Gutzwiller-projected wavefunctions, further improved by Lánczos steps, we demonstrate excellent agreement in both energies and correlation functions between a gapless (Dirac) $\mathbb{Z}_2$ spin liquid-characterized by only a few variational parameters-and results obtained from neural quantum states and DMRG. Finally, we apply the recently developed Keldysh formulation of the pseudo-fermion functional renormalization group to compute the dynamical spin structure factor. The resulting spectra exhibit features consistent with Dirac cones in the excitation spectrum, providing strong independent evidence for a Dirac QSL ground state. Our identification of a $d$-wave pairing $\mathbb{Z}_2$ Dirac QSL is consistent with recently observed signatures of QSL behavior in Pr$_2$Ga$_2$BeO$_7$ and outlines predictions for future experiments.
format Preprint
id arxiv_https___arxiv_org_abs_2501_00096
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Evidence for a $\mathbb{Z}_{2}$ Dirac spin liquid in the generalized Shastry-Sutherland model
Maity, Atanu
Ferrari, Francesco
Capponi, Sylvain
Penc, Karlo
Potten, Janik
Müller, Tobias
Feuerpfeil, Andreas
Thomale, Ronny
Lee, Jong Yeon
Samajdar, Rhine
Iqbal, Yasir
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
We present a multimethod investigation into the nature of the recently reported quantum spin liquid (QSL) phase in the spin-$1/2$ Heisenberg antiferromagnet on the Shastry-Sutherland lattice. A comprehensive projective symmetry group classification of fermionic mean-field Ansätze on this lattice yields 46 U(1) and 80 $\mathbb{Z}_2$ states. Using density-matrix renormalization group (DMRG) and exact diagonalization calculations, we find that the Shastry-Sutherland model and the square-lattice $J_1$-$J_2$ Heisenberg antiferromagnet share the same QSL phase. Motivated by this observation, we establish an explicit mapping of our Ansätze to those on the square lattice, and identify the counterpart of the square-lattice $\mathbb{Z}_2$ Dirac QSL (Z2A$zz$13) in the Shastry-Sutherland system. Employing state-of-the-art variational Monte Carlo calculations with Gutzwiller-projected wavefunctions, further improved by Lánczos steps, we demonstrate excellent agreement in both energies and correlation functions between a gapless (Dirac) $\mathbb{Z}_2$ spin liquid-characterized by only a few variational parameters-and results obtained from neural quantum states and DMRG. Finally, we apply the recently developed Keldysh formulation of the pseudo-fermion functional renormalization group to compute the dynamical spin structure factor. The resulting spectra exhibit features consistent with Dirac cones in the excitation spectrum, providing strong independent evidence for a Dirac QSL ground state. Our identification of a $d$-wave pairing $\mathbb{Z}_2$ Dirac QSL is consistent with recently observed signatures of QSL behavior in Pr$_2$Ga$_2$BeO$_7$ and outlines predictions for future experiments.
title Evidence for a $\mathbb{Z}_{2}$ Dirac spin liquid in the generalized Shastry-Sutherland model
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2501.00096