Self-reconfiguring colloidal active matter

Fuente: arXiv
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Main Authors: Ketzetzi, Stefania, Caprini, Lorenzo, Willems, Vivien, Alvarez, Laura, Löwen, Hartmut, Isa, Lucio
Format: Preprint
Published: 2024
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author Ketzetzi, Stefania
Caprini, Lorenzo
Willems, Vivien
Alvarez, Laura
Löwen, Hartmut
Isa, Lucio
author_facet Ketzetzi, Stefania
Caprini, Lorenzo
Willems, Vivien
Alvarez, Laura
Löwen, Hartmut
Isa, Lucio
contents Cells and microorganisms employ dynamic shape changes to enable steering and avoidance for efficient spatial exploration and collective organization. In contrast, active colloids, their synthetic counterparts, currently lack similar abilities and strategies. Through physical interactions alone, here we create active colloidal molecules that spontaneously reconfigure their structure, unlike traditional active particles. We find that self-reconfiguration decouples reorientational dynamics from rotational diffusivity and bestows our active molecules additional reorientation capabilities. During encounters with neighbors, rapid conformational changes lead to self-steering and avoidance. At higher area fractions, reconfiguration-induced avoidance fully inhibits characteristic dynamic clustering, motility-induced phase separation and flocking; instead, the system retains a homogeneous structure comprising well-separated active units. Self-reconfiguring systems therefore present an exciting path towards autonomous motion beyond that of classical synthetic active matter.
format Preprint
id arxiv_https___arxiv_org_abs_2501_00672
institution arXiv
publishDate 2024
record_format arxiv
spellingShingle Self-reconfiguring colloidal active matter
Ketzetzi, Stefania
Caprini, Lorenzo
Willems, Vivien
Alvarez, Laura
Löwen, Hartmut
Isa, Lucio
Soft Condensed Matter
Cells and microorganisms employ dynamic shape changes to enable steering and avoidance for efficient spatial exploration and collective organization. In contrast, active colloids, their synthetic counterparts, currently lack similar abilities and strategies. Through physical interactions alone, here we create active colloidal molecules that spontaneously reconfigure their structure, unlike traditional active particles. We find that self-reconfiguration decouples reorientational dynamics from rotational diffusivity and bestows our active molecules additional reorientation capabilities. During encounters with neighbors, rapid conformational changes lead to self-steering and avoidance. At higher area fractions, reconfiguration-induced avoidance fully inhibits characteristic dynamic clustering, motility-induced phase separation and flocking; instead, the system retains a homogeneous structure comprising well-separated active units. Self-reconfiguring systems therefore present an exciting path towards autonomous motion beyond that of classical synthetic active matter.
title Self-reconfiguring colloidal active matter
topic Soft Condensed Matter
url https://arxiv.org/abs/2501.00672