Emergence of Giant Magnetic Chirality during Dimensionality Crossover of Magnetic Materials

Fuente: arXiv
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Autori principali: Kim, Dae-Yun, Nam, Yun-Seok, Kim, Younghak, Kim, Kyoung-Whan, Go, Gyungchoon, Lee, Seong-Hyub, Moon, Joon, Chang, Jun-Young, Lee, Ah-Yeon, Park, Seung-Young, Min, Byoung-Chul, Lee, Kyung-Jin, Yang, Hyunsoo, Kim, Duck-Ho, Choe, Sug-Bong
Natura: Preprint
Pubblicazione: 2025
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author Kim, Dae-Yun
Nam, Yun-Seok
Kim, Younghak
Kim, Kyoung-Whan
Go, Gyungchoon
Lee, Seong-Hyub
Moon, Joon
Chang, Jun-Young
Lee, Ah-Yeon
Park, Seung-Young
Min, Byoung-Chul
Lee, Kyung-Jin
Yang, Hyunsoo
Kim, Duck-Ho
Choe, Sug-Bong
author_facet Kim, Dae-Yun
Nam, Yun-Seok
Kim, Younghak
Kim, Kyoung-Whan
Go, Gyungchoon
Lee, Seong-Hyub
Moon, Joon
Chang, Jun-Young
Lee, Ah-Yeon
Park, Seung-Young
Min, Byoung-Chul
Lee, Kyung-Jin
Yang, Hyunsoo
Kim, Duck-Ho
Choe, Sug-Bong
contents Chirality, an intrinsic preference for a specific handedness, is a fundamental characteristic observed in nature. In magnetism, magnetic chirality arises from the anti-symmetric Dzyaloshinskii-Moriya interaction in competition with the symmetric Heisenberg exchange interaction. Traditionally, the anti-symmetric interaction has been considered minor relative to the symmetric interaction. In this study, we demonstrate an observation of giant magnetic chirality during the dimensionality crossover of magnetic materials from three-dimensional to two-dimensional. The ratio between the anti-symmetric and symmetric interactions exhibits a reversal in their dominance over this crossover, overturning the traditional consideration. This observation is validated theoretically using a non-local interaction model and tight-binding calculation with distinct pairing schemes for each exchange interaction throughout the crossover. Additional experiments investigating the asphericity of orbital moments corroborate the robustness of our findings. Our findings highlight the critical role of dimensionality in shaping magnetic chirality and offer strategies for engineering chiral magnet states with unprecedented strength, desired for the design of spintronic materials.
format Preprint
id arxiv_https___arxiv_org_abs_2501_02768
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Emergence of Giant Magnetic Chirality during Dimensionality Crossover of Magnetic Materials
Kim, Dae-Yun
Nam, Yun-Seok
Kim, Younghak
Kim, Kyoung-Whan
Go, Gyungchoon
Lee, Seong-Hyub
Moon, Joon
Chang, Jun-Young
Lee, Ah-Yeon
Park, Seung-Young
Min, Byoung-Chul
Lee, Kyung-Jin
Yang, Hyunsoo
Kim, Duck-Ho
Choe, Sug-Bong
Materials Science
Applied Physics
Chirality, an intrinsic preference for a specific handedness, is a fundamental characteristic observed in nature. In magnetism, magnetic chirality arises from the anti-symmetric Dzyaloshinskii-Moriya interaction in competition with the symmetric Heisenberg exchange interaction. Traditionally, the anti-symmetric interaction has been considered minor relative to the symmetric interaction. In this study, we demonstrate an observation of giant magnetic chirality during the dimensionality crossover of magnetic materials from three-dimensional to two-dimensional. The ratio between the anti-symmetric and symmetric interactions exhibits a reversal in their dominance over this crossover, overturning the traditional consideration. This observation is validated theoretically using a non-local interaction model and tight-binding calculation with distinct pairing schemes for each exchange interaction throughout the crossover. Additional experiments investigating the asphericity of orbital moments corroborate the robustness of our findings. Our findings highlight the critical role of dimensionality in shaping magnetic chirality and offer strategies for engineering chiral magnet states with unprecedented strength, desired for the design of spintronic materials.
title Emergence of Giant Magnetic Chirality during Dimensionality Crossover of Magnetic Materials
topic Materials Science
Applied Physics
url https://arxiv.org/abs/2501.02768