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Autores principales:	Wark, J. S., Peake, D. J., Stevens, T., Heighway, P. G., Ping, Y., Sterne, P., Albertazzi, B., Ali, S. J., Antonelli, L., Armstrong, M. R., Baehtz, C., Ball, O. B., Banerjee, S., Belonoshko, A. B., Bolme, C. A., Bouffetier, V., Briggs, R., Buakor, K., Butcher, T., Cafiso, S. Di Dio, Cerantola, V., Chantel, J., Di Cicco, A., Coleman, A. L., Collier, J., Collins, G., Comley, A. J., Coppari, F., Cowan, T. E., Cristoforetti, G., Cynn, H., Descamps, A., Dorchies, F., Duff, M. J., Dwivedi, A., Edwards, C., Eggert, J. H., Errandonea, D., Fiquet, G., Galtier, E., Garcia, A. Laso, Ginestet, H., Gizzi, L., Gleason, A., Goede, S., Gonzalez, J. M., Gorman, M. G., Harmand, M., Hartley, N., Hernandez-Gomez, C., Higginbotham, A., Höppner, H., Humphries, O. S., Husband, R. J., Hutchinson, T. M., Hwang, H., Keen, D. A., Kim, J., Koester, P., Konopkova, Z., Kraus, D., Krygier, A., Labate, L., Lazicki, A. E., Lee, Y., Liermann, H-P., Mason, P., Masruri, M., Massani, B., McBride, E. E., McGuire, C., McHardy, J. D., McGonegle, D., McWilliams, R. S., Merkel, S., Morard, G., Nagler, B., Nakatsutsumi, M., Nguyen-Cong, K., Norton, A-M., Oleynik, I. I., Otzen, C., Ozaki, N., Pandolfi, S., Pelka, A., Pereira, K. A., Phillips, J. P., Prescher, C., Preston, T., Randolph, L., Ranjan, D., Ravasio, A., Redmer, R., Rips, J., Santamaria-Perez, D., Savage, D. J., Schoelmerich, M., Schwinkendorf, J-P., Singh, S., Smith, J., Smith, R. F., Sollier, A., Spear, J., Spindloe, C., Stevenson, M., Strohm, C., Suer, T-A., Tang, M., Toncian, M., Toncian, T., Tracy, S. J., Trapananti, A., Tschentscher, T., Tyldesley, M., Vennari, C. E., Vinci, T., Vogel, S. C., Volz, T. J., Vorberger, J., Willman, J. T., Wollenweber, L., Zastrau, U., Brambrink, E., Appel, K., McMahon, M. I.
Formato:	Preprint
Publicado:	2025
Materias:	Materials Science Applied Physics
Acceso en línea:	https://arxiv.org/abs/2501.02940
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author	Wark, J. S. Peake, D. J. Stevens, T. Heighway, P. G. Ping, Y. Sterne, P. Albertazzi, B. Ali, S. J. Antonelli, L. Armstrong, M. R. Baehtz, C. Ball, O. B. Banerjee, S. Belonoshko, A. B. Bolme, C. A. Bouffetier, V. Briggs, R. Buakor, K. Butcher, T. Cafiso, S. Di Dio Cerantola, V. Chantel, J. Di Cicco, A. Coleman, A. L. Collier, J. Collins, G. Comley, A. J. Coppari, F. Cowan, T. E. Cristoforetti, G. Cynn, H. Descamps, A. Dorchies, F. Duff, M. J. Dwivedi, A. Edwards, C. Eggert, J. H. Errandonea, D. Fiquet, G. Galtier, E. Garcia, A. Laso Ginestet, H. Gizzi, L. Gleason, A. Goede, S. Gonzalez, J. M. Gorman, M. G. Harmand, M. Hartley, N. Hernandez-Gomez, C. Higginbotham, A. Höppner, H. Humphries, O. S. Husband, R. J. Hutchinson, T. M. Hwang, H. Keen, D. A. Kim, J. Koester, P. Konopkova, Z. Kraus, D. Krygier, A. Labate, L. Lazicki, A. E. Lee, Y. Liermann, H-P. Mason, P. Masruri, M. Massani, B. McBride, E. E. McGuire, C. McHardy, J. D. McGonegle, D. McWilliams, R. S. Merkel, S. Morard, G. Nagler, B. Nakatsutsumi, M. Nguyen-Cong, K. Norton, A-M. Oleynik, I. I. Otzen, C. Ozaki, N. Pandolfi, S. Pelka, A. Pereira, K. A. Phillips, J. P. Prescher, C. Preston, T. Randolph, L. Ranjan, D. Ravasio, A. Redmer, R. Rips, J. Santamaria-Perez, D. Savage, D. J. Schoelmerich, M. Schwinkendorf, J-P. Singh, S. Smith, J. Smith, R. F. Sollier, A. Spear, J. Spindloe, C. Stevenson, M. Strohm, C. Suer, T-A. Tang, M. Toncian, M. Toncian, T. Tracy, S. J. Trapananti, A. Tschentscher, T. Tyldesley, M. Vennari, C. E. Vinci, T. Vogel, S. C. Volz, T. J. Vorberger, J. Willman, J. T. Wollenweber, L. Zastrau, U. Brambrink, E. Appel, K. McMahon, M. I.
author_facet	Wark, J. S. Peake, D. J. Stevens, T. Heighway, P. G. Ping, Y. Sterne, P. Albertazzi, B. Ali, S. J. Antonelli, L. Armstrong, M. R. Baehtz, C. Ball, O. B. Banerjee, S. Belonoshko, A. B. Bolme, C. A. Bouffetier, V. Briggs, R. Buakor, K. Butcher, T. Cafiso, S. Di Dio Cerantola, V. Chantel, J. Di Cicco, A. Coleman, A. L. Collier, J. Collins, G. Comley, A. J. Coppari, F. Cowan, T. E. Cristoforetti, G. Cynn, H. Descamps, A. Dorchies, F. Duff, M. J. Dwivedi, A. Edwards, C. Eggert, J. H. Errandonea, D. Fiquet, G. Galtier, E. Garcia, A. Laso Ginestet, H. Gizzi, L. Gleason, A. Goede, S. Gonzalez, J. M. Gorman, M. G. Harmand, M. Hartley, N. Hernandez-Gomez, C. Higginbotham, A. Höppner, H. Humphries, O. S. Husband, R. J. Hutchinson, T. M. Hwang, H. Keen, D. A. Kim, J. Koester, P. Konopkova, Z. Kraus, D. Krygier, A. Labate, L. Lazicki, A. E. Lee, Y. Liermann, H-P. Mason, P. Masruri, M. Massani, B. McBride, E. E. McGuire, C. McHardy, J. D. McGonegle, D. McWilliams, R. S. Merkel, S. Morard, G. Nagler, B. Nakatsutsumi, M. Nguyen-Cong, K. Norton, A-M. Oleynik, I. I. Otzen, C. Ozaki, N. Pandolfi, S. Pelka, A. Pereira, K. A. Phillips, J. P. Prescher, C. Preston, T. Randolph, L. Ranjan, D. Ravasio, A. Redmer, R. Rips, J. Santamaria-Perez, D. Savage, D. J. Schoelmerich, M. Schwinkendorf, J-P. Singh, S. Smith, J. Smith, R. F. Sollier, A. Spear, J. Spindloe, C. Stevenson, M. Strohm, C. Suer, T-A. Tang, M. Toncian, M. Toncian, T. Tracy, S. J. Trapananti, A. Tschentscher, T. Tyldesley, M. Vennari, C. E. Vinci, T. Vogel, S. C. Volz, T. J. Vorberger, J. Willman, J. T. Wollenweber, L. Zastrau, U. Brambrink, E. Appel, K. McMahon, M. I.
contents	We present 50-fs, single-shot measurements of the x-ray thermal diffuse scattering (TDS) from copper foils that have been shocked via nanosecond laser-ablation up to pressures above 135~GPa. We hence deduce the x-ray Debye-Waller (DW) factor, providing a temperature measurement. The targets were laser-shocked with the DiPOLE 100-X laser at the High Energy Density (HED) endstation of the European X-ray Free-Electron Laser (EuXFEL). Single x-ray pulses, with a photon energy of 18 keV, were scattered from the samples and recorded on Varex detectors. Despite the targets being highly textured (as evinced by large variations in the elastic scattering), and with such texture changing upon compression, the absolute intensity of the azimuthally averaged inelastic TDS between the Bragg peaks is largely insensitive to these changes, and, allowing for both Compton scattering and the low-level scattering from a sacrificial ablator layer, provides a reliable measurement of $T/Θ_D^2$, where $Θ_D$ is the Debye temperature. We compare our results with the predictions of the SESAME 3336 and LEOS 290 equations of state for copper, and find good agreement within experimental errors. We thus demonstrate that single-shot temperature measurements of dynamically compressed materials can be made via thermal diffuse scattering of XFEL radation.
format	Preprint
id	arxiv_https___arxiv_org_abs_2501_02940
institution	arXiv
publishDate	2025
record_format	arxiv
spellingShingle	Femtosecond temperature measurements of laser-shocked copper deduced from the intensity of the x-ray thermal diffuse scattering Wark, J. S. Peake, D. J. Stevens, T. Heighway, P. G. Ping, Y. Sterne, P. Albertazzi, B. Ali, S. J. Antonelli, L. Armstrong, M. R. Baehtz, C. Ball, O. B. Banerjee, S. Belonoshko, A. B. Bolme, C. A. Bouffetier, V. Briggs, R. Buakor, K. Butcher, T. Cafiso, S. Di Dio Cerantola, V. Chantel, J. Di Cicco, A. Coleman, A. L. Collier, J. Collins, G. Comley, A. J. Coppari, F. Cowan, T. E. Cristoforetti, G. Cynn, H. Descamps, A. Dorchies, F. Duff, M. J. Dwivedi, A. Edwards, C. Eggert, J. H. Errandonea, D. Fiquet, G. Galtier, E. Garcia, A. Laso Ginestet, H. Gizzi, L. Gleason, A. Goede, S. Gonzalez, J. M. Gorman, M. G. Harmand, M. Hartley, N. Hernandez-Gomez, C. Higginbotham, A. Höppner, H. Humphries, O. S. Husband, R. J. Hutchinson, T. M. Hwang, H. Keen, D. A. Kim, J. Koester, P. Konopkova, Z. Kraus, D. Krygier, A. Labate, L. Lazicki, A. E. Lee, Y. Liermann, H-P. Mason, P. Masruri, M. Massani, B. McBride, E. E. McGuire, C. McHardy, J. D. McGonegle, D. McWilliams, R. S. Merkel, S. Morard, G. Nagler, B. Nakatsutsumi, M. Nguyen-Cong, K. Norton, A-M. Oleynik, I. I. Otzen, C. Ozaki, N. Pandolfi, S. Pelka, A. Pereira, K. A. Phillips, J. P. Prescher, C. Preston, T. Randolph, L. Ranjan, D. Ravasio, A. Redmer, R. Rips, J. Santamaria-Perez, D. Savage, D. J. Schoelmerich, M. Schwinkendorf, J-P. Singh, S. Smith, J. Smith, R. F. Sollier, A. Spear, J. Spindloe, C. Stevenson, M. Strohm, C. Suer, T-A. Tang, M. Toncian, M. Toncian, T. Tracy, S. J. Trapananti, A. Tschentscher, T. Tyldesley, M. Vennari, C. E. Vinci, T. Vogel, S. C. Volz, T. J. Vorberger, J. Willman, J. T. Wollenweber, L. Zastrau, U. Brambrink, E. Appel, K. McMahon, M. I. Materials Science Applied Physics We present 50-fs, single-shot measurements of the x-ray thermal diffuse scattering (TDS) from copper foils that have been shocked via nanosecond laser-ablation up to pressures above 135~GPa. We hence deduce the x-ray Debye-Waller (DW) factor, providing a temperature measurement. The targets were laser-shocked with the DiPOLE 100-X laser at the High Energy Density (HED) endstation of the European X-ray Free-Electron Laser (EuXFEL). Single x-ray pulses, with a photon energy of 18 keV, were scattered from the samples and recorded on Varex detectors. Despite the targets being highly textured (as evinced by large variations in the elastic scattering), and with such texture changing upon compression, the absolute intensity of the azimuthally averaged inelastic TDS between the Bragg peaks is largely insensitive to these changes, and, allowing for both Compton scattering and the low-level scattering from a sacrificial ablator layer, provides a reliable measurement of $T/Θ_D^2$, where $Θ_D$ is the Debye temperature. We compare our results with the predictions of the SESAME 3336 and LEOS 290 equations of state for copper, and find good agreement within experimental errors. We thus demonstrate that single-shot temperature measurements of dynamically compressed materials can be made via thermal diffuse scattering of XFEL radation.
title	Femtosecond temperature measurements of laser-shocked copper deduced from the intensity of the x-ray thermal diffuse scattering
topic	Materials Science Applied Physics
url	https://arxiv.org/abs/2501.02940

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