Single-molecule Scale Magnetic Resonance Spectroscopy using Nitrogen-Vacancy Centers in Diamond

Fuente: arXiv
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Autori principali: Du, Jiangfeng, Shi, Fazhan, Kong, Xi, Jekezko, Fedor, Wrachtrup, Jörg
Natura: Preprint
Pubblicazione: 2025
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author Du, Jiangfeng
Shi, Fazhan
Kong, Xi
Jekezko, Fedor
Wrachtrup, Jörg
author_facet Du, Jiangfeng
Shi, Fazhan
Kong, Xi
Jekezko, Fedor
Wrachtrup, Jörg
contents Single-molecule technology stands as a powerful tool, enabling the characterization of intricate structural and dynamic information that would otherwise remain concealed within the averaged behaviors of numerous molecules. This technology finds extensive application across diverse fields including physics, chemistry, biology, and medicine. Quantum sensing, particularly leveraging nitrogen-vacancy (NV) centers within diamond structures, presents a promising avenue for single-molecule magnetic resonance, offering prospects for sensing and imaging technology at the single-molecule level. Notably, while significant strides have been made in single-molecule scale magnetic resonance using NV centers over the past two decades, current approaches still exhibit limitations in magnetic sensitivity, spectral resolution, and spatial resolution. Particularly, the full reconstruction of three-dimensional positions of nuclear spins within single molecules remains an unattained goal. This review provides a comprehensive overview of the current state-of-the-art in single-molecule scale magnetic resonance, encompassing an analysis of various relevant techniques involving NV centers. Additionally, it explores the optimization of technical parameters associated with these methods. This detailed analysis serves as a foundation for the development of new technologies and the exploration of potential applications.
format Preprint
id arxiv_https___arxiv_org_abs_2501_03620
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Single-molecule Scale Magnetic Resonance Spectroscopy using Nitrogen-Vacancy Centers in Diamond
Du, Jiangfeng
Shi, Fazhan
Kong, Xi
Jekezko, Fedor
Wrachtrup, Jörg
Quantum Physics
Mesoscale and Nanoscale Physics
Applied Physics
Instrumentation and Detectors
Single-molecule technology stands as a powerful tool, enabling the characterization of intricate structural and dynamic information that would otherwise remain concealed within the averaged behaviors of numerous molecules. This technology finds extensive application across diverse fields including physics, chemistry, biology, and medicine. Quantum sensing, particularly leveraging nitrogen-vacancy (NV) centers within diamond structures, presents a promising avenue for single-molecule magnetic resonance, offering prospects for sensing and imaging technology at the single-molecule level. Notably, while significant strides have been made in single-molecule scale magnetic resonance using NV centers over the past two decades, current approaches still exhibit limitations in magnetic sensitivity, spectral resolution, and spatial resolution. Particularly, the full reconstruction of three-dimensional positions of nuclear spins within single molecules remains an unattained goal. This review provides a comprehensive overview of the current state-of-the-art in single-molecule scale magnetic resonance, encompassing an analysis of various relevant techniques involving NV centers. Additionally, it explores the optimization of technical parameters associated with these methods. This detailed analysis serves as a foundation for the development of new technologies and the exploration of potential applications.
title Single-molecule Scale Magnetic Resonance Spectroscopy using Nitrogen-Vacancy Centers in Diamond
topic Quantum Physics
Mesoscale and Nanoscale Physics
Applied Physics
Instrumentation and Detectors
url https://arxiv.org/abs/2501.03620