Spectroscopy of the Fractal Hofstadter Energy Spectrum

Fuente: arXiv
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Autori principali: Nuckolls, Kevin P., Scheer, Michael G., Wong, Dillon, Oh, Myungchul, Lee, Ryan L., Herzog-Arbeitman, Jonah, Watanabe, Kenji, Taniguchi, Takashi, Lian, Biao, Yazdani, Ali
Natura: Preprint
Pubblicazione: 2025
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author Nuckolls, Kevin P.
Scheer, Michael G.
Wong, Dillon
Oh, Myungchul
Lee, Ryan L.
Herzog-Arbeitman, Jonah
Watanabe, Kenji
Taniguchi, Takashi
Lian, Biao
Yazdani, Ali
author_facet Nuckolls, Kevin P.
Scheer, Michael G.
Wong, Dillon
Oh, Myungchul
Lee, Ryan L.
Herzog-Arbeitman, Jonah
Watanabe, Kenji
Taniguchi, Takashi
Lian, Biao
Yazdani, Ali
contents Hofstadter's butterfly, the predicted energy spectrum for non-interacting electrons confined to a two-dimensional lattice in a magnetic field, is one of the most remarkable fractal structures in nature. At rational ratios of magnetic flux quanta per lattice unit cell, this spectrum shows self-similar distributions of energy levels that reflect its recursive construction. For most materials, Hofstadter's butterfly is predicted under experimental conditions that are unachievable using laboratory-scale magnetic fields. More recently, electrical transport studies have provided evidence for Hofstadter's butterfly in materials engineered to have artificially large lattice constants, such as those with moiré superlattices. Yet to-date, direct spectroscopy of the fractal energy spectrum predicted by Hofstadter nearly 50 years ago has remained out of reach. Here we use high-resolution scanning tunneling microscopy / spectroscopy (STM / STS) to probe the flat electronic bands in twisted bilayer graphene near the predicted second magic angle, an ideal setting for spectroscopic studies of Hofstadter's spectrum. Our study shows the fractionalization of flat moiré bands into discrete Hofstadter subbands and discerns experimental signatures of self-similarity of this spectrum. Moreover, our measurements uncover a spectrum that evolves dynamically with electron density, displaying phenomena beyond that of Hofstadter's original model due to the combined effects of strong correlations, Coulomb interactions, and the quantum degeneracy of electrons in twisted bilayer graphene.
format Preprint
id arxiv_https___arxiv_org_abs_2501_04777
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Spectroscopy of the Fractal Hofstadter Energy Spectrum
Nuckolls, Kevin P.
Scheer, Michael G.
Wong, Dillon
Oh, Myungchul
Lee, Ryan L.
Herzog-Arbeitman, Jonah
Watanabe, Kenji
Taniguchi, Takashi
Lian, Biao
Yazdani, Ali
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
Hofstadter's butterfly, the predicted energy spectrum for non-interacting electrons confined to a two-dimensional lattice in a magnetic field, is one of the most remarkable fractal structures in nature. At rational ratios of magnetic flux quanta per lattice unit cell, this spectrum shows self-similar distributions of energy levels that reflect its recursive construction. For most materials, Hofstadter's butterfly is predicted under experimental conditions that are unachievable using laboratory-scale magnetic fields. More recently, electrical transport studies have provided evidence for Hofstadter's butterfly in materials engineered to have artificially large lattice constants, such as those with moiré superlattices. Yet to-date, direct spectroscopy of the fractal energy spectrum predicted by Hofstadter nearly 50 years ago has remained out of reach. Here we use high-resolution scanning tunneling microscopy / spectroscopy (STM / STS) to probe the flat electronic bands in twisted bilayer graphene near the predicted second magic angle, an ideal setting for spectroscopic studies of Hofstadter's spectrum. Our study shows the fractionalization of flat moiré bands into discrete Hofstadter subbands and discerns experimental signatures of self-similarity of this spectrum. Moreover, our measurements uncover a spectrum that evolves dynamically with electron density, displaying phenomena beyond that of Hofstadter's original model due to the combined effects of strong correlations, Coulomb interactions, and the quantum degeneracy of electrons in twisted bilayer graphene.
title Spectroscopy of the Fractal Hofstadter Energy Spectrum
topic Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
url https://arxiv.org/abs/2501.04777