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Main Authors: Grasdijk, Olivier, DeMille, David, Kastelic, Jakob, Kawall, David, Lamoreaux, Steve, Timgren, Oskari, Wenz, Konrad, Zelevinsky, Tanya
Format: Preprint
Published: 2025
Subjects:
Online Access:https://arxiv.org/abs/2501.05578
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author Grasdijk, Olivier
DeMille, David
Kastelic, Jakob
Kawall, David
Lamoreaux, Steve
Timgren, Oskari
Wenz, Konrad
Zelevinsky, Tanya
author_facet Grasdijk, Olivier
DeMille, David
Kastelic, Jakob
Kawall, David
Lamoreaux, Steve
Timgren, Oskari
Wenz, Konrad
Zelevinsky, Tanya
contents The aim of CeNTREX (Cold Molecule Nuclear Time-Reversal Experiment) is to search for time-reversal symmetry violation in the thallium nucleus, by measuring the Schiff moment of $^{205}$Tl in the polar molecule thallium fluoride (TlF). CeNTREX uses a cryogenic beam of TlF with a rotational temperature of 6.3(2) K. This results in population spread over dozens of rotational and hyperfine sublevels of TlF, while only a single level is useful for the Schiff moment measurement. Here we present a protocol for cooling the rotational and hyperfine degrees of freedom in the CeNTREX beam, transferring the majority of the Boltzmann distribution into a single rotational and hyperfine sublevel by using a single ultraviolet laser and a pair of microwave beams. We achieve a factor of $20.1(4)$ gain in the population of the $J=0$, $F=0$ hyperfine sublevel of the TlF ground state.
format Preprint
id arxiv_https___arxiv_org_abs_2501_05578
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Rotational-hyperfine cooling of $^{205}$TlF in a cryogenic beam
Grasdijk, Olivier
DeMille, David
Kastelic, Jakob
Kawall, David
Lamoreaux, Steve
Timgren, Oskari
Wenz, Konrad
Zelevinsky, Tanya
Atomic Physics
The aim of CeNTREX (Cold Molecule Nuclear Time-Reversal Experiment) is to search for time-reversal symmetry violation in the thallium nucleus, by measuring the Schiff moment of $^{205}$Tl in the polar molecule thallium fluoride (TlF). CeNTREX uses a cryogenic beam of TlF with a rotational temperature of 6.3(2) K. This results in population spread over dozens of rotational and hyperfine sublevels of TlF, while only a single level is useful for the Schiff moment measurement. Here we present a protocol for cooling the rotational and hyperfine degrees of freedom in the CeNTREX beam, transferring the majority of the Boltzmann distribution into a single rotational and hyperfine sublevel by using a single ultraviolet laser and a pair of microwave beams. We achieve a factor of $20.1(4)$ gain in the population of the $J=0$, $F=0$ hyperfine sublevel of the TlF ground state.
title Rotational-hyperfine cooling of $^{205}$TlF in a cryogenic beam
topic Atomic Physics
url https://arxiv.org/abs/2501.05578