Weak electronic correlations in the cobalt oxychalcogenide superconductor Na2CoSe2O

Fuente: arXiv
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Autori principali: Wu, Zhenchao, Cao, Yingying, Luo, Hong-Gang, Yang, Yi-feng
Natura: Preprint
Pubblicazione: 2025
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author Wu, Zhenchao
Cao, Yingying
Luo, Hong-Gang
Yang, Yi-feng
author_facet Wu, Zhenchao
Cao, Yingying
Luo, Hong-Gang
Yang, Yi-feng
contents Motivated by the newly discovered Co-based superconductor Na2CoSe2O, we performed systematic calculations of its electronic band structures using the density functional theory (DFT) plus the dynamical mean-field theory (DMFT) approaches. Our comparative studies reveal weakly correlated and itinerant nature of the Co-3d electrons and show no sign of fluctuating local moments as expected in many other unconventional superconductors, although the Co eg orbitals are close to half filling. These suggest that Na2CoSe2O is a normal paramagnetic metal and its superconductivity might not be of strongly correlated nature, contrary to the initial speculation. We suggest future investigations of electron-phonon interactions to clarify its pairing mechanism.
format Preprint
id arxiv_https___arxiv_org_abs_2501_09675
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Weak electronic correlations in the cobalt oxychalcogenide superconductor Na2CoSe2O
Wu, Zhenchao
Cao, Yingying
Luo, Hong-Gang
Yang, Yi-feng
Strongly Correlated Electrons
Superconductivity
Motivated by the newly discovered Co-based superconductor Na2CoSe2O, we performed systematic calculations of its electronic band structures using the density functional theory (DFT) plus the dynamical mean-field theory (DMFT) approaches. Our comparative studies reveal weakly correlated and itinerant nature of the Co-3d electrons and show no sign of fluctuating local moments as expected in many other unconventional superconductors, although the Co eg orbitals are close to half filling. These suggest that Na2CoSe2O is a normal paramagnetic metal and its superconductivity might not be of strongly correlated nature, contrary to the initial speculation. We suggest future investigations of electron-phonon interactions to clarify its pairing mechanism.
title Weak electronic correlations in the cobalt oxychalcogenide superconductor Na2CoSe2O
topic Strongly Correlated Electrons
Superconductivity
url https://arxiv.org/abs/2501.09675