Electrically tunable Floquet Weyl photon emission from Dirac semimetal Cd3As2

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Hauptverfasser: Mishra, Sobhan Subhra, Tan, Thomas CaiWei, Gupta, Manoj, Xiu, Faxian, Singh, Ranjan
Format: Preprint
Veröffentlicht: 2025
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author Mishra, Sobhan Subhra
Tan, Thomas CaiWei
Gupta, Manoj
Xiu, Faxian
Singh, Ranjan
author_facet Mishra, Sobhan Subhra
Tan, Thomas CaiWei
Gupta, Manoj
Xiu, Faxian
Singh, Ranjan
contents The ability to optically engineer the Dirac band and electrically control the Fermi level in two-dimensional (2D) Dirac systems, such as graphene, has significantly advanced quantum technologies. However, similar tunability has remained elusive in three-dimensional Dirac systems. In this work, we demonstrate both optical and electrical tunability of the band structure in the 3D Dirac semimetal Cd3As2. Photoexcitation with circularly polarized light breaks time-reversal symmetry, lifting the degeneracy at Dirac points to transform the material into a Floquet Weyl semimetal with chiral Weyl nodes. This transition induces nonzero Berry curvature, giving rise to helicity-dependent transverse anomalous photocurrents, detectable through terahertz emission at normal incidence. Furthermore, applying an external electric field displaces the Fermi level away from the Dirac point, enlarging the Dirac cone projection leading to a reduced density of states of Fermi arcs. As a result, we achieve precise electrical control over Floquet band engineering, resulting in a large modulation of THz emission. Moreover, at oblique incidence, the circular photon-drag effect induces helicity-dependent longitudinal photocurrents. Simultaneous generation and manipulation of both longitudinal and transverse photocurrents enable precise control of the helicity of emitted THz pulses. These results pave the way for electric field-controlled Floquet Weyl THz sources, offering significant potential for applications in quantum computing and low-power electronics.
format Preprint
id arxiv_https___arxiv_org_abs_2501_16498
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Electrically tunable Floquet Weyl photon emission from Dirac semimetal Cd3As2
Mishra, Sobhan Subhra
Tan, Thomas CaiWei
Gupta, Manoj
Xiu, Faxian
Singh, Ranjan
Materials Science
The ability to optically engineer the Dirac band and electrically control the Fermi level in two-dimensional (2D) Dirac systems, such as graphene, has significantly advanced quantum technologies. However, similar tunability has remained elusive in three-dimensional Dirac systems. In this work, we demonstrate both optical and electrical tunability of the band structure in the 3D Dirac semimetal Cd3As2. Photoexcitation with circularly polarized light breaks time-reversal symmetry, lifting the degeneracy at Dirac points to transform the material into a Floquet Weyl semimetal with chiral Weyl nodes. This transition induces nonzero Berry curvature, giving rise to helicity-dependent transverse anomalous photocurrents, detectable through terahertz emission at normal incidence. Furthermore, applying an external electric field displaces the Fermi level away from the Dirac point, enlarging the Dirac cone projection leading to a reduced density of states of Fermi arcs. As a result, we achieve precise electrical control over Floquet band engineering, resulting in a large modulation of THz emission. Moreover, at oblique incidence, the circular photon-drag effect induces helicity-dependent longitudinal photocurrents. Simultaneous generation and manipulation of both longitudinal and transverse photocurrents enable precise control of the helicity of emitted THz pulses. These results pave the way for electric field-controlled Floquet Weyl THz sources, offering significant potential for applications in quantum computing and low-power electronics.
title Electrically tunable Floquet Weyl photon emission from Dirac semimetal Cd3As2
topic Materials Science
url https://arxiv.org/abs/2501.16498