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Main Authors: Ladbrook, Evie, Dey, Urmimala, Bristowe, Nicholas C., Perry, Robin S., Daisenberger, Dominik, Warren, Mark R., Senn, Mark S.
Format: Preprint
Published: 2025
Subjects:
Online Access:https://arxiv.org/abs/2501.18728
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author Ladbrook, Evie
Dey, Urmimala
Bristowe, Nicholas C.
Perry, Robin S.
Daisenberger, Dominik
Warren, Mark R.
Senn, Mark S.
author_facet Ladbrook, Evie
Dey, Urmimala
Bristowe, Nicholas C.
Perry, Robin S.
Daisenberger, Dominik
Warren, Mark R.
Senn, Mark S.
contents Polar metals are an intriguing class of materials in which electric polarisation and metallicity can coexist within a single phase. The unique properties of polar metals challenge expectations, making way for the exploration of exotic phenomena such as unconventional magnetism, hyperferroelectric multiferroicity and developing multifunctional devices that can leverage both the materials electric polarization and its asymmetry in the spin conductivity, that arises due to the Rashba effect. Here, via a high pressure single crystal diffraction study, we report the pressure-induced enhancement of polar distortions in such a metal, Ca$_3$Ru$_2$O$_7$. Our DFT calculations highlight that naive assumptions about the linear dependency between polar distortion amplitudes and the magnitude of the Rashba spin splitting may not be generally valid.
format Preprint
id arxiv_https___arxiv_org_abs_2501_18728
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Pressure induced enhancement of polar distortions in a metal, and implications on the Rashba spin-splitting
Ladbrook, Evie
Dey, Urmimala
Bristowe, Nicholas C.
Perry, Robin S.
Daisenberger, Dominik
Warren, Mark R.
Senn, Mark S.
Strongly Correlated Electrons
Materials Science
Polar metals are an intriguing class of materials in which electric polarisation and metallicity can coexist within a single phase. The unique properties of polar metals challenge expectations, making way for the exploration of exotic phenomena such as unconventional magnetism, hyperferroelectric multiferroicity and developing multifunctional devices that can leverage both the materials electric polarization and its asymmetry in the spin conductivity, that arises due to the Rashba effect. Here, via a high pressure single crystal diffraction study, we report the pressure-induced enhancement of polar distortions in such a metal, Ca$_3$Ru$_2$O$_7$. Our DFT calculations highlight that naive assumptions about the linear dependency between polar distortion amplitudes and the magnitude of the Rashba spin splitting may not be generally valid.
title Pressure induced enhancement of polar distortions in a metal, and implications on the Rashba spin-splitting
topic Strongly Correlated Electrons
Materials Science
url https://arxiv.org/abs/2501.18728