Strong geometry dependence of the X-ray Thomson Scattering Spectrum in single crystal silicon

Fuente: arXiv
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Autores principales: Gawne, Thomas, Moldabekov, Zhandos A., Humphries, Oliver S., Appel, Karen, Baehtz, Carsten, Bouffetier, Victorien, Brambrink, Erik, Cangi, Attila, Crépisson, Celine, Göde, Sebastian, Konôpková, Zuzana, Makita, Mikako, Mishchenko, Mikhail, Nakatsutsumi, Motoaki, Randolph, Lisa, Schwalbe, Sebastian, Vorberger, Jan, Zastrau, Ulf, Dornheim, Tobias, Preston, Thomas R.
Formato: Preprint
Publicado: 2025
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author Gawne, Thomas
Moldabekov, Zhandos A.
Humphries, Oliver S.
Appel, Karen
Baehtz, Carsten
Bouffetier, Victorien
Brambrink, Erik
Cangi, Attila
Crépisson, Celine
Göde, Sebastian
Konôpková, Zuzana
Makita, Mikako
Mishchenko, Mikhail
Nakatsutsumi, Motoaki
Randolph, Lisa
Schwalbe, Sebastian
Vorberger, Jan
Zastrau, Ulf
Dornheim, Tobias
Preston, Thomas R.
author_facet Gawne, Thomas
Moldabekov, Zhandos A.
Humphries, Oliver S.
Appel, Karen
Baehtz, Carsten
Bouffetier, Victorien
Brambrink, Erik
Cangi, Attila
Crépisson, Celine
Göde, Sebastian
Konôpková, Zuzana
Makita, Mikako
Mishchenko, Mikhail
Nakatsutsumi, Motoaki
Randolph, Lisa
Schwalbe, Sebastian
Vorberger, Jan
Zastrau, Ulf
Dornheim, Tobias
Preston, Thomas R.
contents We report on results from an experiment at the European XFEL where we measured the x-ray Thomson scattering (XRTS) spectrum of single crystal silicon with ultrahigh resolution. Compared to similar previous experiments, we consider a more complex scattering setup, in which the scattering vector changes orientation through the crystal lattice. In doing so, we are able to observe strong geometric dependencies in the inelastic scattering spectrum of silicon at low scattering angles. Furthermore, the high quality of the experimental data allows us to benchmark state-of-the-art TDDFT calculations, and demonstrate TDDFT's ability to accurately predict these geometric dependencies. Finally, we note that this experimental data was collected at a much faster rate than another recently reported dataset using the same setup, demonstrating that ultrahigh resolution XRTS data can be collected in more general experimental scenarios.
format Preprint
id arxiv_https___arxiv_org_abs_2501_19276
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Strong geometry dependence of the X-ray Thomson Scattering Spectrum in single crystal silicon
Gawne, Thomas
Moldabekov, Zhandos A.
Humphries, Oliver S.
Appel, Karen
Baehtz, Carsten
Bouffetier, Victorien
Brambrink, Erik
Cangi, Attila
Crépisson, Celine
Göde, Sebastian
Konôpková, Zuzana
Makita, Mikako
Mishchenko, Mikhail
Nakatsutsumi, Motoaki
Randolph, Lisa
Schwalbe, Sebastian
Vorberger, Jan
Zastrau, Ulf
Dornheim, Tobias
Preston, Thomas R.
Materials Science
Plasma Physics
We report on results from an experiment at the European XFEL where we measured the x-ray Thomson scattering (XRTS) spectrum of single crystal silicon with ultrahigh resolution. Compared to similar previous experiments, we consider a more complex scattering setup, in which the scattering vector changes orientation through the crystal lattice. In doing so, we are able to observe strong geometric dependencies in the inelastic scattering spectrum of silicon at low scattering angles. Furthermore, the high quality of the experimental data allows us to benchmark state-of-the-art TDDFT calculations, and demonstrate TDDFT's ability to accurately predict these geometric dependencies. Finally, we note that this experimental data was collected at a much faster rate than another recently reported dataset using the same setup, demonstrating that ultrahigh resolution XRTS data can be collected in more general experimental scenarios.
title Strong geometry dependence of the X-ray Thomson Scattering Spectrum in single crystal silicon
topic Materials Science
Plasma Physics
url https://arxiv.org/abs/2501.19276