Generation of photon pairs through spontaneous four-wave mixing in subwavelength nonlinear films

Fuente: arXiv
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Autores principales: Son, Changjin, Peana, Samuel, Matthiessen, Owen, Kryvobok, Artem, Senichev, Alexander, Boltasseva, Alexandra, Shalaev, Vladimir M., Chekhova, Maria
Formato: Preprint
Publicado: 2025
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author Son, Changjin
Peana, Samuel
Matthiessen, Owen
Kryvobok, Artem
Senichev, Alexander
Boltasseva, Alexandra
Shalaev, Vladimir M.
Chekhova, Maria
author_facet Son, Changjin
Peana, Samuel
Matthiessen, Owen
Kryvobok, Artem
Senichev, Alexander
Boltasseva, Alexandra
Shalaev, Vladimir M.
Chekhova, Maria
contents Pairs of entangled photons are crucial for photonic quantum technologies. The demand for integrability and multi-functionality suggests 'flat' platforms - ultrathin layers and metasurfaces - as sources of photon pairs. Despite the success in the demonstration of spontaneous parametric down-conversion (SPDC) from such sources, there are almost no works on spontaneous four-wave mixing (SFWM) - an alternative process to generate photon pairs. Meanwhile, SFWM can be implemented in any nanostructures, including ones made of isotropic materials, which are easier to fabricate than crystalline SPDC sources. Here, we investigate photon pair generation through SFWM in subwavelength films of amorphous silicon nitride (SiN) with varying nitrogen content. For all samples, we demonstrate two-photon quantum correlations, indicated by the normalized second-order correlation function g(2)(0): it exceeds 2 and decays as the pump power increases. By observing two-photon interference between SFWM from the SiN films and the fused silica substrate, we find the third-order susceptibilities of films with different nitrogen content.
format Preprint
id arxiv_https___arxiv_org_abs_2502_01305
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Generation of photon pairs through spontaneous four-wave mixing in subwavelength nonlinear films
Son, Changjin
Peana, Samuel
Matthiessen, Owen
Kryvobok, Artem
Senichev, Alexander
Boltasseva, Alexandra
Shalaev, Vladimir M.
Chekhova, Maria
Optics
Quantum Physics
Pairs of entangled photons are crucial for photonic quantum technologies. The demand for integrability and multi-functionality suggests 'flat' platforms - ultrathin layers and metasurfaces - as sources of photon pairs. Despite the success in the demonstration of spontaneous parametric down-conversion (SPDC) from such sources, there are almost no works on spontaneous four-wave mixing (SFWM) - an alternative process to generate photon pairs. Meanwhile, SFWM can be implemented in any nanostructures, including ones made of isotropic materials, which are easier to fabricate than crystalline SPDC sources. Here, we investigate photon pair generation through SFWM in subwavelength films of amorphous silicon nitride (SiN) with varying nitrogen content. For all samples, we demonstrate two-photon quantum correlations, indicated by the normalized second-order correlation function g(2)(0): it exceeds 2 and decays as the pump power increases. By observing two-photon interference between SFWM from the SiN films and the fused silica substrate, we find the third-order susceptibilities of films with different nitrogen content.
title Generation of photon pairs through spontaneous four-wave mixing in subwavelength nonlinear films
topic Optics
Quantum Physics
url https://arxiv.org/abs/2502.01305