Easy-cone state mediating the spin reorientation in topological kagome magnet Fe$_3$Sn$_2$

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Auteurs principaux: Prodan, L., Evans, D. M., Sukhanov, A. S., Nikitin, S. E., Tsirlin, A. A., Puntingam, L., Rahn, M. C., Chioncel, L., Tsurkan, V., Kezsmarki, I.
Format: Preprint
Publié: 2025
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author Prodan, L.
Evans, D. M.
Sukhanov, A. S.
Nikitin, S. E.
Tsirlin, A. A.
Puntingam, L.
Rahn, M. C.
Chioncel, L.
Tsurkan, V.
Kezsmarki, I.
author_facet Prodan, L.
Evans, D. M.
Sukhanov, A. S.
Nikitin, S. E.
Tsirlin, A. A.
Puntingam, L.
Rahn, M. C.
Chioncel, L.
Tsurkan, V.
Kezsmarki, I.
contents We investigated temperature-driven spin reorientation (SR) in the itinerant kagome magnet Fe$_3$Sn$_2$ using high-resolution synchrotron x-ray diffraction, neutron diffraction, magnetometry, and magnetic force microscopy (MFM), further supported by phenomenological analysis. Our study reveals a crossover from the state with easy-plane anisotropy to the high-temperature state with uniaxial easy-axis anisotropy taking place between $\sim40-130$~ K through an intermediate easy-cone (or tilted spin) state. This state, induced by the interplay between the anisotropy constants $K_1$ and $K_2$, is clearly manifested in the thermal evolution of the magnetic structure factor, which reveals a gradual change of the SR angle $\mathbfθ$ between $40-130$~K. We also found that the SR is accompanied by a magnetoelastic effect. Zero-field MFM images across the SR range show a transformation in surface magnetic patterns from a dendritic structure at 120~K, to domain wall dominated MFM contrast at 40~K.
format Preprint
id arxiv_https___arxiv_org_abs_2502_03239
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Easy-cone state mediating the spin reorientation in topological kagome magnet Fe$_3$Sn$_2$
Prodan, L.
Evans, D. M.
Sukhanov, A. S.
Nikitin, S. E.
Tsirlin, A. A.
Puntingam, L.
Rahn, M. C.
Chioncel, L.
Tsurkan, V.
Kezsmarki, I.
Materials Science
Strongly Correlated Electrons
We investigated temperature-driven spin reorientation (SR) in the itinerant kagome magnet Fe$_3$Sn$_2$ using high-resolution synchrotron x-ray diffraction, neutron diffraction, magnetometry, and magnetic force microscopy (MFM), further supported by phenomenological analysis. Our study reveals a crossover from the state with easy-plane anisotropy to the high-temperature state with uniaxial easy-axis anisotropy taking place between $\sim40-130$~ K through an intermediate easy-cone (or tilted spin) state. This state, induced by the interplay between the anisotropy constants $K_1$ and $K_2$, is clearly manifested in the thermal evolution of the magnetic structure factor, which reveals a gradual change of the SR angle $\mathbfθ$ between $40-130$~K. We also found that the SR is accompanied by a magnetoelastic effect. Zero-field MFM images across the SR range show a transformation in surface magnetic patterns from a dendritic structure at 120~K, to domain wall dominated MFM contrast at 40~K.
title Easy-cone state mediating the spin reorientation in topological kagome magnet Fe$_3$Sn$_2$
topic Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2502.03239