Photoemission electron microscopy of exciton-polaritons in thin WSe$_2$ waveguides

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Hauptverfasser: Eul, Tobias, Sabir, Miwan, DeManuel-Gonzalez, Victor, Diekmann, Florian, Rossnagel, Kai, Bauer, Michael
Format: Preprint
Veröffentlicht: 2025
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author Eul, Tobias
Sabir, Miwan
DeManuel-Gonzalez, Victor
Diekmann, Florian
Rossnagel, Kai
Bauer, Michael
author_facet Eul, Tobias
Sabir, Miwan
DeManuel-Gonzalez, Victor
Diekmann, Florian
Rossnagel, Kai
Bauer, Michael
contents Exciton-polaritons emerging from the interaction of photons and excitons in the strong coupling regime are intriguing quasiparticles for the potential exchange of energy during light-matter interaction processes such as light harvesting. The coupling causes an energy anti-crossing in the photon dispersion centered around the exciton resonance, i.e., a Rabi splitting between a lower and upper energetic branch. The size of this splitting correlates with the coupling strength between the exciton and the photonic modes. In this work, we investigate this coupling between excitons and photonic waveguide modes excited simultaneously in thin-film flakes of the transition-metal dichalcogenide WSe$_2$. Using a Photoemission electron microscope, we are able to extract the dispersion of the transversal electric and magnetic modes propagating through these flakes as well as extract the energy splitting. Ultimately, our findings provide a basis for the investigation of the propagation of exciton-polaritons in the time-domain via time-resolved photoemission.
format Preprint
id arxiv_https___arxiv_org_abs_2502_03361
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Photoemission electron microscopy of exciton-polaritons in thin WSe$_2$ waveguides
Eul, Tobias
Sabir, Miwan
DeManuel-Gonzalez, Victor
Diekmann, Florian
Rossnagel, Kai
Bauer, Michael
Materials Science
Exciton-polaritons emerging from the interaction of photons and excitons in the strong coupling regime are intriguing quasiparticles for the potential exchange of energy during light-matter interaction processes such as light harvesting. The coupling causes an energy anti-crossing in the photon dispersion centered around the exciton resonance, i.e., a Rabi splitting between a lower and upper energetic branch. The size of this splitting correlates with the coupling strength between the exciton and the photonic modes. In this work, we investigate this coupling between excitons and photonic waveguide modes excited simultaneously in thin-film flakes of the transition-metal dichalcogenide WSe$_2$. Using a Photoemission electron microscope, we are able to extract the dispersion of the transversal electric and magnetic modes propagating through these flakes as well as extract the energy splitting. Ultimately, our findings provide a basis for the investigation of the propagation of exciton-polaritons in the time-domain via time-resolved photoemission.
title Photoemission electron microscopy of exciton-polaritons in thin WSe$_2$ waveguides
topic Materials Science
url https://arxiv.org/abs/2502.03361