Pressure suppresses the density wave order in kagome metal LuNb$_6$Sn$_6$

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Hauptverfasser: Meier, William R., Graf, David E., Ortiz, Brenden R., Mozaffari, Shirin, Mandrus, David
Format: Preprint
Veröffentlicht: 2025
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author Meier, William R.
Graf, David E.
Ortiz, Brenden R.
Mozaffari, Shirin
Mandrus, David
author_facet Meier, William R.
Graf, David E.
Ortiz, Brenden R.
Mozaffari, Shirin
Mandrus, David
contents Dancing tins pair up, But compressing the framework Thwarts the displacements. The density waves that develop in kagome metals ScV$_{6}$Sn$_{6}$ and LuNb$_{6}$Sn$_{6}$ at low temperature appear to arise from under-filled atomic columns within a V-Sn or Nb-Sn scaffolding. Compressing this network with applied pressure in ScV$_{6}$Sn$_{6}$ suppressed the structural transition temperature by constraining atomic rattling and inhibiting the shifts that define the structural modulation. We predicted that the density wave transition in LuNb$_{6}$Sn$_{6}$ at 68 K would be suppressed by pressure as well. In this brief study, we examine the pressure dependence of the density wave transition by measuring resistance vs temperature up to 2.26 GPa. We found the transition temperature is smoothly depressed and disappears around 1.9 GPa. This result not only addresses our prediction, but strengthens the rattling chains origin of structural instabilities in the HfFe$_{6}$Ge$_{6}$-type kagome metals.
format Preprint
id arxiv_https___arxiv_org_abs_2502_04197
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Pressure suppresses the density wave order in kagome metal LuNb$_6$Sn$_6$
Meier, William R.
Graf, David E.
Ortiz, Brenden R.
Mozaffari, Shirin
Mandrus, David
Strongly Correlated Electrons
Dancing tins pair up, But compressing the framework Thwarts the displacements. The density waves that develop in kagome metals ScV$_{6}$Sn$_{6}$ and LuNb$_{6}$Sn$_{6}$ at low temperature appear to arise from under-filled atomic columns within a V-Sn or Nb-Sn scaffolding. Compressing this network with applied pressure in ScV$_{6}$Sn$_{6}$ suppressed the structural transition temperature by constraining atomic rattling and inhibiting the shifts that define the structural modulation. We predicted that the density wave transition in LuNb$_{6}$Sn$_{6}$ at 68 K would be suppressed by pressure as well. In this brief study, we examine the pressure dependence of the density wave transition by measuring resistance vs temperature up to 2.26 GPa. We found the transition temperature is smoothly depressed and disappears around 1.9 GPa. This result not only addresses our prediction, but strengthens the rattling chains origin of structural instabilities in the HfFe$_{6}$Ge$_{6}$-type kagome metals.
title Pressure suppresses the density wave order in kagome metal LuNb$_6$Sn$_6$
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2502.04197