Microscopic description of quadrupole-hexadecapole coupling in radium, thorium, uranium and plutonium isotopes with the Gogny energy density functional

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Hauptverfasser: Rodriguez-Guzman, R., Robledo, L. M.
Format: Preprint
Veröffentlicht: 2025
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author Rodriguez-Guzman, R.
Robledo, L. M.
author_facet Rodriguez-Guzman, R.
Robledo, L. M.
contents The emergence and stability of static hexadecapole deformations as well as the impact in the development of dynamic deformation due to collective motion considering quadrupole-hexadecapole coupling are studied for a selected set of radium, thorium, uranium and plutonium isotopes, using the Gogny Hartree-Fock-Bogoliubov and Generator Coordinate Method frameworks. Sizable hexadecapole deformations are found to play a significant role in the ground and excited states of nuclei in the neighborhood of $^{238}$U. For each of the studied isotopic chains, it is shown that a region with small negative hexadecapole deformation, just below the neutron magic number $N =184$, remains stable once zero-point quadrupole-hexadecapole fluctuations are taken into account. A transition is predicted, with increasing mass number, from a regime in which the quadrupole and hexadecapole degrees of freedom are interwoven to a regime in which they are decoupled, accompanied by an enhanced shape coexistence in the more neutron-rich sectors of the isotopic chains. It is also shown, that quadrupole-hexadecapole configuration mixing brings a nontrivial additional correlation energy gain comparable to the quadrupole correlation energy itself.
format Preprint
id arxiv_https___arxiv_org_abs_2502_04985
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Microscopic description of quadrupole-hexadecapole coupling in radium, thorium, uranium and plutonium isotopes with the Gogny energy density functional
Rodriguez-Guzman, R.
Robledo, L. M.
Nuclear Theory
The emergence and stability of static hexadecapole deformations as well as the impact in the development of dynamic deformation due to collective motion considering quadrupole-hexadecapole coupling are studied for a selected set of radium, thorium, uranium and plutonium isotopes, using the Gogny Hartree-Fock-Bogoliubov and Generator Coordinate Method frameworks. Sizable hexadecapole deformations are found to play a significant role in the ground and excited states of nuclei in the neighborhood of $^{238}$U. For each of the studied isotopic chains, it is shown that a region with small negative hexadecapole deformation, just below the neutron magic number $N =184$, remains stable once zero-point quadrupole-hexadecapole fluctuations are taken into account. A transition is predicted, with increasing mass number, from a regime in which the quadrupole and hexadecapole degrees of freedom are interwoven to a regime in which they are decoupled, accompanied by an enhanced shape coexistence in the more neutron-rich sectors of the isotopic chains. It is also shown, that quadrupole-hexadecapole configuration mixing brings a nontrivial additional correlation energy gain comparable to the quadrupole correlation energy itself.
title Microscopic description of quadrupole-hexadecapole coupling in radium, thorium, uranium and plutonium isotopes with the Gogny energy density functional
topic Nuclear Theory
url https://arxiv.org/abs/2502.04985