Strong coupling between a dielectric nanocavity and a monolayer transition metal dichalcogenide

Fuente: arXiv
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Autores principales: Schröder, F., Wyborski, P., Xiong, M., Kountouris, G., Munkhbat, B., Wubs, M., Kristensen, P. T., Mørk, J., Stenger, N.
Formato: Preprint
Publicado: 2025
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author Schröder, F.
Wyborski, P.
Xiong, M.
Kountouris, G.
Munkhbat, B.
Wubs, M.
Kristensen, P. T.
Mørk, J.
Stenger, N.
author_facet Schröder, F.
Wyborski, P.
Xiong, M.
Kountouris, G.
Munkhbat, B.
Wubs, M.
Kristensen, P. T.
Mørk, J.
Stenger, N.
contents We demonstrate strong coupling between light in a dielectric nanocavity with deep sub-wavelength confinement and excitons in a monolayer of molybdenum ditelluride. Avoided crossing is demonstrated by both photoluminescence and reflection measurements, from which we extract a light-matter interaction strength of $g_{\mathrm{PL}} =\SI{5.3\pm0.3}{\milli\eV}$ and $g_{\mathrm{R}} =\SI{4.7\pm0.7}{\milli\eV}$, respectively. The associated Rabi splitting is twice as large as the system's losses. These values are in good agreement with values obtained by a novel exciton reaction coordinate formalism, yielding $g_{\mathrm{theory}} = \SI{5.2\pm0.7}{\milli\eV}$. The strong light-matter interaction, combined with low losses and sub-wavelength confinement of light, black demonstrates a new regime of light-matter interactions where strong nonlinearities at the single-photon level are expected.
format Preprint
id arxiv_https___arxiv_org_abs_2502_06529
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Strong coupling between a dielectric nanocavity and a monolayer transition metal dichalcogenide
Schröder, F.
Wyborski, P.
Xiong, M.
Kountouris, G.
Munkhbat, B.
Wubs, M.
Kristensen, P. T.
Mørk, J.
Stenger, N.
Optics
Other Condensed Matter
We demonstrate strong coupling between light in a dielectric nanocavity with deep sub-wavelength confinement and excitons in a monolayer of molybdenum ditelluride. Avoided crossing is demonstrated by both photoluminescence and reflection measurements, from which we extract a light-matter interaction strength of $g_{\mathrm{PL}} =\SI{5.3\pm0.3}{\milli\eV}$ and $g_{\mathrm{R}} =\SI{4.7\pm0.7}{\milli\eV}$, respectively. The associated Rabi splitting is twice as large as the system's losses. These values are in good agreement with values obtained by a novel exciton reaction coordinate formalism, yielding $g_{\mathrm{theory}} = \SI{5.2\pm0.7}{\milli\eV}$. The strong light-matter interaction, combined with low losses and sub-wavelength confinement of light, black demonstrates a new regime of light-matter interactions where strong nonlinearities at the single-photon level are expected.
title Strong coupling between a dielectric nanocavity and a monolayer transition metal dichalcogenide
topic Optics
Other Condensed Matter
url https://arxiv.org/abs/2502.06529