Emergence of Order in Chemically Active Droplets: Temporal Dynamics and Collective Behavior

Fuente: arXiv
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Autori principali: Ashraf, Sobiya, Kumar, Pawan, Dwivedi, Prateek, Blanc, Frédéric, Pillai, Dipin, Mangal, Rahul
Natura: Preprint
Pubblicazione: 2025
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author Ashraf, Sobiya
Kumar, Pawan
Dwivedi, Prateek
Blanc, Frédéric
Pillai, Dipin
Mangal, Rahul
author_facet Ashraf, Sobiya
Kumar, Pawan
Dwivedi, Prateek
Blanc, Frédéric
Pillai, Dipin
Mangal, Rahul
contents Collective behaviors such as swarming, chemical signaling, and clustering are fundamental to biological microorganisms, enabling hierarchical colony formation, coordinated motion, and enhanced nutrient accessibility crucial for their survival. Over the past few decades, extensive research has been dedicated to unraveling the mechanisms underlying these diverse collective patterns through experimental model systems. Among these, active droplets have emerged as valuable synthetic analogs, effectively replicating key biological attributes and serving as ideal platforms for investigating collective phenomena. This research explores the collective behavior of 4-Cyano-4-pentyl-biphenyl (5CB) oil droplets across varying Péclet ($Pe$) numbers. At high $Pe$, droplets exhibit a pusher mode of propulsion and form dynamic chain-like patterns. Decreasing $Pe$ enhances repulsive interactions among droplets, resulting in the inhibition of clustering. In the low $Pe$ regime, their repulsive interactions predominated by chemical field lead to the emergence of an ordered structure. Furthermore, we illustrate how active droplets efficiently navigate within a soft structured environment. These findings contribute to our comprehension of self-organized phenomena in active matter systems and provide insights for designing strategies for controlled locomotion in intricate fluidic environments.
format Preprint
id arxiv_https___arxiv_org_abs_2502_07009
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Emergence of Order in Chemically Active Droplets: Temporal Dynamics and Collective Behavior
Ashraf, Sobiya
Kumar, Pawan
Dwivedi, Prateek
Blanc, Frédéric
Pillai, Dipin
Mangal, Rahul
Soft Condensed Matter
Collective behaviors such as swarming, chemical signaling, and clustering are fundamental to biological microorganisms, enabling hierarchical colony formation, coordinated motion, and enhanced nutrient accessibility crucial for their survival. Over the past few decades, extensive research has been dedicated to unraveling the mechanisms underlying these diverse collective patterns through experimental model systems. Among these, active droplets have emerged as valuable synthetic analogs, effectively replicating key biological attributes and serving as ideal platforms for investigating collective phenomena. This research explores the collective behavior of 4-Cyano-4-pentyl-biphenyl (5CB) oil droplets across varying Péclet ($Pe$) numbers. At high $Pe$, droplets exhibit a pusher mode of propulsion and form dynamic chain-like patterns. Decreasing $Pe$ enhances repulsive interactions among droplets, resulting in the inhibition of clustering. In the low $Pe$ regime, their repulsive interactions predominated by chemical field lead to the emergence of an ordered structure. Furthermore, we illustrate how active droplets efficiently navigate within a soft structured environment. These findings contribute to our comprehension of self-organized phenomena in active matter systems and provide insights for designing strategies for controlled locomotion in intricate fluidic environments.
title Emergence of Order in Chemically Active Droplets: Temporal Dynamics and Collective Behavior
topic Soft Condensed Matter
url https://arxiv.org/abs/2502.07009